Citation: Yuxiang Wang, Yutong Xu, Weiwei Zeng, Xinxing Zhan, Jinliang Zhuang, Yuan-Zhi Tan. Electrocatalytic carbon materials derived from fullerene pyrolysis[J]. Chinese Chemical Letters, ;2026, 37(12): 112819. doi: 10.1016/j.cclet.2026.112819 shu

Electrocatalytic carbon materials derived from fullerene pyrolysis

Yuxiang Wang ^a ,
Yutong Xu ^a ,
Weiwei Zeng ^a ,
Xinxing Zhan ^b ,
Jinliang Zhuang ^{b, *,} ,
Yuan-Zhi Tan ^{a, *,}

a.
State Key Laboratory of Physical Chemistry of Solid Surfaces, and Department of Chemistry, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China
b.
School of Chemistry and Materials Science, Key Lab for Functional Materials, Chemistry of Guizhou Province, Guizhou Normal University, Guiyang 550025, China

jlzhuang@xmu.edu.cn

yuanzhi_tan@xmu.edu.cn

Received Date: 28 December 2025
Revised Date: 18 April 2026
Accepted Date: 21 April 2026
Available Online: 24 April 2026

Figures(11)

Carbon nanomaterials have emerged as promising electrocatalysts for sustainable energy storage and conversion. As a unique allotrope, fullerenes offer distinct advantages, including high reactivity and a highly curved structure. However, their electrocatalytic application is limited by inherently low electrical conductivity, limited specific surface area, and insufficient intrinsic activity. Pyrolytic transformation of fullerenes provides an effective strategy to overcome these limitations, yielding carbon materials that are rich in defects, feature porous architectures with high surface areas, and possess tunable surface chemistry. These attributes meet the critical requirements for electrocatalysis—abundant active sites and efficient mass/charge transport—establishing pyrolyzed fullerene-derived carbons as a highly promising platform for advanced electrocatalysis. This review summarizes the structural evolution mechanisms during pyrolysis, the advantages of the resulting carbons, and their characterization methods. It then analyzes key modification strategies, such as hierarchical engineering, heteroatom doping, and metal composites, to clarify the structure-performance relationships. The representative applications and performance of these derived carbon materials in diverse electrocatalytic reactions are then highlighted. Finally, future opportunities and core challenges are discussed, providing scientific guidance for the rational design of next-generation electrocatalysts from pyrolyzed fullerenes.
- Pyrolyzed fullerene-derived carbons,
- Hierarchical structural engineering,
- Heteroatom doping,
- Metal composites,
- Electrocatalysis
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沈阳化工大学材料科学与工程学院沈阳 110142