Citation: Zhitong Ma, Yuanfang Wang, Yajiao Wang, Xunli Wang, Qingbai Tian, Xing Xu, Hanghang Zhao. MXene-based single-atom catalysis for enhanced Fenton-like reactions in water treatment[J]. Chinese Chemical Letters, ;2026, 37(8): 112721. doi: 10.1016/j.cclet.2026.112721 shu

MXene-based single-atom catalysis for enhanced Fenton-like reactions in water treatment

Zhitong Ma ^a ,
Yuanfang Wang ^{b, *,} ,
Yajiao Wang ^c ,
Xunli Wang ^c ,
Qingbai Tian ^d ,
Xing Xu ^{d, *,} ,
Hanghang Zhao ^{c, *,}

a.
College of Geology and Environment, Xi’an University of Science and Technology, Xi’an 710054, China
b.
Department of Chemistry and Chemical & Environmental Engineering, Weifang University, Weifang 261061, China
c.
School of Chemical and Environment Science, Shaanxi University of Technology, Hanzhong 723001, China
d.
Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Qingdao 266237, China

20160024@wfu.edu.cn

xuxing@sdu.edu.cn

zhaohh931106@163.com

Received Date: 31 January 2026
Revised Date: 25 March 2026
Accepted Date: 2 April 2026
Available Online: 3 April 2026

Figures(5)

The application of MXene-based single-atom catalysts (SACs) in Fenton-like processes has emerged as a rapidly advancing research frontier in recent years. Early studies have demonstrated their superior activity in activating peroxymonosulfate or hydrogen peroxide for pollutant degradation compared to conventional nanoparticle catalysts, while recent efforts have shifted toward precise structural engineering and mechanistic understanding of reaction pathways. However, the transition from laboratory-scale synthesis to industrial implementation remains challenging, due to difficulties in developing green and scalable fabrication methods, long-term instability in complex water matrices, leaching of metal active centers, and the lack of cost-effective integration into continuous-flow systems such as fixed-bed reactors. To date, comprehensive reviews addressing their engineering applications remain limited. This review systematically summarizes advances in synthetic strategies and characterization techniques for achieving atomic dispersion, elucidates the structure–activity relationships and synergistic radical/non-radical mechanisms, and evaluates reactor design and scale-up potential. Particular emphasis is placed on operational adaptability and economic feasibility under real-world conditions. Future perspectives include the rational design of novel MXene supports, machine learning-assisted catalyst optimization, hybrid process integration, and the development of sustainability assessment frameworks, aiming to bridge the gap between fundamental discoveries and practical water purification technologies.
- MXenes,
- Single-atom catalysis,
- Fenton-like system,
- Catalytic devices,
- Pollutants
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沈阳化工大学材料科学与工程学院沈阳 110142