Citation: Zhimin Yuan, Xingling Zhao, Xianglin Zhu, Kaili Wang, Ya-Qian Lan, Zaiyong Jiang. Solar-driven hydrogen peroxide production on designed g-C₃N₄: Strategies, mechanisms, and perspectives[J]. Chinese Chemical Letters, ;2026, 37(6): 112572. doi: 10.1016/j.cclet.2026.112572 shu

Solar-driven hydrogen peroxide production on designed g-C₃N₄: Strategies, mechanisms, and perspectives

Zhimin Yuan ^a ,
Xingling Zhao ^a ,
Xianglin Zhu ^{c, *,} ,
Kaili Wang ^a ,
Ya-Qian Lan ^{b, *,} ,
Zaiyong Jiang ^{a, *,}

a.
School of Chemistry & Chemical Engineering and Environmental Engineering, Weifang University, Weifang 261061, China
b.
School of Chemistry, South China Normal University, Guangzhou 510006, China
c.
Institute for Energy Research, Jiangsu University, Zhenjiang 212013, China

zhuxl@ujs.edu.cn

yqlan@m.scnu.edu.cn

zaiyongjiang@qlu.edu.cn

Received Date: 13 December 2025
Revised Date: 24 February 2026
Accepted Date: 2 March 2026
Available Online: 6 March 2026

Figures(10)

The photocatalytic production of hydrogen peroxide (H₂O₂) utilizing graphitic carbon nitride (g-C₃N₄) offers a sustainable alternative to the conventional, energy-intensive anthraquinone method. Nevertheless, the practical deployment of pristine g-C₃N₄ is constrained by its limited absorption of visible light, rapid recombination of photogenerated charge carriers, and low surface catalytic activity. This review critically examines various modification strategies aimed at enhancing the H₂O₂ generation efficiency of g-C₃N₄-based photocatalysts. Prominent approaches encompass elemental doping, defect modification, and the junction engineering. These modifications synergistically enhance light absorption, facilitate charge separation, and accelerate oxygen reduction reaction kinetics. Consequently, such engineered photocatalysts have achieved H₂O₂ production rates reaching millimolar concentrations per hour under visible-light irradiation, alongside marked improvements in selectivity and apparent quantum efficiency. Despite these significant advancements, challenges persist in realizing broad-spectrum solar energy utilization, ensuring long-term operational stability, and developing scalable synthesis methods for catalyst fabrication. This review delineates prospective research directions aimed at advancing efficient and practical photocatalytic systems for sustainable hydrogen peroxide synthesis.
- g-C₃N₄-based photocatalysts,
- Hydrogen peroxide production,
- Photocatalytic,
- Modification strategies,
- H₂O₂
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Solar-driven hydrogen peroxide production on designed g-C3N4: Strategies, mechanisms, and perspectives

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Solar-driven hydrogen peroxide production on designed g-C₃N₄: Strategies, mechanisms, and perspectives