Citation: Yue Yin, Yaping Fan, Jiao Yang, Yi Ren, Bo Lai. Structural engineering of piezocatalysts for piezo-driven H₂O₂ production: Enabling multifunctional integration in advanced wastewater remediation[J]. Chinese Chemical Letters, ;2026, 37(10): 112556. doi: 10.1016/j.cclet.2026.112556 shu

Structural engineering of piezocatalysts for piezo-driven H₂O₂ production: Enabling multifunctional integration in advanced wastewater remediation

Yue Yin ^{a, b} ,
Yaping Fan ^{a, b} ,
Jiao Yang ^{a, b, *,} ,
Yi Ren ^{c, *,} ,
Bo Lai ^d

a.
School of Ecology and Environment, Zhengzhou University, Zhengzhou 450001, China
b.
Henan International Joint Laboratory of Environment and Resources, Zhengzhou 450001, China
c.
State Key Laboratory of Hydraulics and Mountain River Engineering, College of Water Resource & Hydropower, Sichuan University, Chengdu 610065, China
d.
State Key Laboratory of Hydraulics and Mountain River Engineering, College of Architecture and Environment, Sichuan University, Chengdu 610065, China

jiaoyang@zzu.edu.cn

yren@scu.edu.cn

Received Date: 4 July 2025
Revised Date: 6 February 2026
Accepted Date: 26 February 2026
Available Online: 27 February 2026

Figures(8)

Piezocatalysis based on electrode polarization processes represents a highly promising approach for in-situ H₂O₂ generation. The efficiency of piezocatalytic H₂O₂ generation faces dual constraints from extrinsic operational parameters like excitation frequency and intrinsic material properties, particularly crystallographic characteristics and polarization magnitude governing charge separation kinetics. Consequently, structural optimization targeting enhanced polarization response, accelerated charge transfer, and strengthened reactant adsorption at active sites has become a central research imperative. This review evaluates piezoelectric material design strategies, establishes structure-function relationships spanning multiscale features and H₂O₂ production efficiency, and assesses technological viability for advanced wastewater remediation. By systematically analyzing core structural determinants, including crystal symmetry, heterojunction, surface functionalization, polymerization degree, and microstructural parameters (porosity/thickness), across diverse piezocatalytic systems, we elucidate governing structure-function interdependencies for H₂O₂ production. These determinants have been further validated in material classes spanning perovskites, bismuth-based layered compounds, wurtzite-type materials, transition metal dichalcogenides, carbon-based materials, polymers, metal-organic frameworks, and MAX phase materials. These insights will establish mechanistic foundations for in-situ H₂O₂ synthesis, advancing sustainable water remediation via piezocatalysis.
- Piezocatalysis,
- H₂O production,
- Structure-function relationships,
- Structural engineering,
- Wastewater remediation
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沈阳化工大学材料科学与工程学院沈阳 110142

Structural engineering of piezocatalysts for piezo-driven H2O2 production: Enabling multifunctional integration in advanced wastewater remediation

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通讯作者: 陈斌, bchen63@163.com

Structural engineering of piezocatalysts for piezo-driven H₂O₂ production: Enabling multifunctional integration in advanced wastewater remediation