Citation: Sai Bai, Qianyu Pan, Xiangning Xu, Minxian Cheng, Xiaoming Peng, Jin Qian. Application of heteroatom-doped carbon in peroxymonosulfate activation for enhancing Fenton-like performance: Current development, challenges and prospects[J]. Chinese Chemical Letters, ;2026, 37(10): 112502. doi: 10.1016/j.cclet.2026.112502 shu

Application of heteroatom-doped carbon in peroxymonosulfate activation for enhancing Fenton-like performance: Current development, challenges and prospects

Sai Bai ^a ,
Qianyu Pan ^b ,
Xiangning Xu ^c ,
Minxian Cheng ^a ,
Xiaoming Peng ^{b, *,} ,
Jin Qian ^{a, *,}

a.
Research & Development Institute in Shenzhen, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi'an 710072, China
b.
School of Civil Engineering and Architecture, East China Jiaotong University, Nanchang 330013, China
c.
The Second Geological Brigade of Sichuan, Chengdu 610081, China

pengxiaoming70@126.com

qianjin@nwpu.edu.cn

Received Date: 22 July 2025
Revised Date: 7 January 2026
Accepted Date: 5 February 2026
Available Online: 7 February 2026

Figures(6)

Emerging contaminants (ECs) present significant environmental and health risks due to their widespread impact. Catalytic Fenton-like reactions using carbon-based catalysts offer a promising and sustainable solution for EC removal. This review synthesizes recent advancements in heteroatom-doped carbon (HDC) catalysts for peroxymonosulfate (PMS) activation, critically evaluating the merits and limitations of HDC-mediated Fenton-like reactions. The review explores how doping affects catalyst porosity, electronic properties, PMS activation efficiency, and overall effectiveness in EC removal. Innovative strategies for identifying key reactive species in HDC/PMS systems are discussed, including the use of chemical probes, spin-trapping agents, and SETP-based methodologies. Additionally, density functional theory (DFT) is utilized to investigate the electronic structures of ECs and their interactions with reactive oxygen species (ROS). The practical potential of HDCs in remediating contaminated groundwater and wastewater is also addressed, alongside a discussion of the challenges and future research directions to enhance their scalable applications, offering a roadmap for advancing sustainable environmental remediation technologies.
- Carbon-based catalysts,
- Peroxymonosulfate,
- Organic pollutants,
- Heteroatom-doping,
- Electronic density
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沈阳化工大学材料科学与工程学院沈阳 110142