Citation: Qianyu Pan, Chuqiao Wang, Caihua Liu, Chong-Chen Wang, Yuying Hu, Xing Xu, Xiaoming Peng. Oxidative polymerization in heterogeneous Fenton-like systems: Towards sustainable water treatment[J]. Chinese Chemical Letters, ;2026, 37(7): 112191. doi: 10.1016/j.cclet.2025.112191 shu

Oxidative polymerization in heterogeneous Fenton-like systems: Towards sustainable water treatment

Qianyu Pan ^a ,
Chuqiao Wang ^a ,
Caihua Liu ^a ,
Chong-Chen Wang ^{b, *,} ,
Yuying Hu ^a ,
Xing Xu ^c ,
Xiaoming Peng ^{a, *,}

a.
School of Civil Engineering and Architecture, East China Jiaotong University, Nanchang 330013, China
b.
Institute of Advanced Materials, Beijing Key Laboratory of Functional Materials for Building Structure and Environment Remediation, Beijing University of Civil Engineering and Architecture, Beijing 100044, China
c.
School of Environmental Science and Engineering, Shandong University, Qingdao 266237, China

wangchongchen@bucea.edu.cn

pengxiaoming70@ecjtu.edu.cn

Received Date: 25 May 2025
Revised Date: 3 November 2025
Accepted Date: 26 November 2025
Available Online: 27 November 2025

Figures(5)

In heterogeneous Fenton-like systems, the oxidative polymerization pathway is of great significance in the field of sustainable water treatment. Unlike the traditional mineralization pathway, it can convert organic pollutants into polymers, thereby achieving the recovery of carbon resources. This paper focuses on the core content related to this pathway, expounding that the mechanism of oxidative polymerization is influenced by multiple factors (catalysts, oxidants, organic matters). Meanwhile, various methods exist for identifying the polymerization pathway, such as electrochemical experiments, Raman spectroscopy analysis, and mass spectrometry technology, which can infer the reaction process and product structure. Additionally, this paper reveals two pathways for pollutant removal through oxidative polymerization: The radical pathway and the non-radical pathway. In the future, advanced characterization techniques should be used to deeply explore the microscopic mechanism of oxidative polymerization, optimize catalyst design, expand practical application research, and explore comprehensive utilization pathways for its products, so as to promote the development of sustainable water treatment technologies.
- Heterogeneous Fenton-like systems,
- Polymerization reactions,
- Pollutant removal pathways,
- Radical/non-radical,
- Sustainable water purification
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