Citation: Yingjin Li, Jiaming Li, Hongjun Dong, Wenli Zhang, Liqiu Zhang, Xiulian Yin, Yun Wang, Zuoyi Liu, Chunmei Li. Recent research progress on metal-organic frameworks and their derivatives heterostructure for photocatalytic CO₂ reduction[J]. Chinese Chemical Letters, ;2026, 37(6): 112101. doi: 10.1016/j.cclet.2025.112101 shu

Recent research progress on metal-organic frameworks and their derivatives heterostructure for photocatalytic CO₂ reduction

Yingjin Li ^a ,
Jiaming Li ^a ,
Hongjun Dong ^{a, *,} ,
Wenli Zhang ^a ,
Liqiu Zhang ^{b, *,} ,
Xiulian Yin ^a ,
Yun Wang ^a ,
Zuoyi Liu ^{c, *,} ,
Chunmei Li ^{a, *,}

a.
Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, China
b.
College of Biological, Chemical Sciences and Engineering, Jiaxing University, Jiaxing 314001, China
c.
South China Institute of Environmental Sciences, Ministry of Ecology and Environment. Guangzhou 51000, China

hjdong@ujs.edu.cn

liqiu0524@zjxu.edu.cn

liuzuoyi@scies.org

lichun_mei_happy@126.com

Received Date: 22 August 2025
Revised Date: 10 November 2025
Accepted Date: 11 November 2025
Available Online: 13 November 2025

Figures(22)

Metal-organic frameworks (MOFs) and their derivatives have emerged as promising platforms for constructing heterojunctions in photocatalytic CO₂ reduction (PCR). This review systematically summarizes the latest research progress in MOFs and their derivative heterostructures for PCR, focusing on material design, underlying mechanisms, and diverse applications. Besides, this review, by introducing various synthesis methods, emphasizes the significance of controllable synthesis strategies. Furthermore, the in-situ characterization techniques and theoretical calculations in photocatalysis are introduced and summarized, including the study of the morphology and chemical structure of photocatalysts, the transfer of photogenerated charges, spatial distribution, and surface reaction pathways. Systematic reviews of the advantages and disadvantages, features, and applications of various types of MOFs and their derivative heterostructures are conducted in accordance with the band arrangement characteristics. In addition, the discussion scope is expanded to related catalytic systems, including electrocatalysis, photoelectrocatalysis, and photothermal catalysis, fully demonstrating the multifunctionality of MOFs and their derivative heterostructures. Finally, future research directions are proposed from aspects such as material design and synthesis, performance optimization and mechanism research, correlation with practical applications, as well as the interdisciplinary collaboration. We hope it can provide valuable references for the rational design of high-performance MOFs and their derivative heterostructures materials with the wide range of applications.
- Metal-organic frameworks,
- Heterostructure,
- Co₂ reduction,
- Photocatalysis,
- In-situ characterization techniques,
- Mechanism
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沈阳化工大学材料科学与工程学院沈阳 110142

Recent research progress on metal-organic frameworks and their derivatives heterostructure for photocatalytic CO2 reduction

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通讯作者: 陈斌, bchen63@163.com

Recent research progress on metal-organic frameworks and their derivatives heterostructure for photocatalytic CO₂ reduction