Citation: Zihui Liu, Xiaolin Liu, Lin Tang, Houhe Pan, Xi Liu, Jianzhuang Jiang. Covalent organic frameworks-based heterojunctions for photocatalytic hydrogen peroxide production and in-situ application[J]. Chinese Chemical Letters, ;2026, 37(6): 112024. doi: 10.1016/j.cclet.2025.112024 shu

Covalent organic frameworks-based heterojunctions for photocatalytic hydrogen peroxide production and in-situ application

Zihui Liu ^a ,
Xiaolin Liu ^{a, *,} ,
Lin Tang ^a ,
Houhe Pan ^{b, *,} ,
Xi Liu ^{a, *,} ,
Jianzhuang Jiang ^{b, c, *,}

a.
Chongqing Key Laboratory of Green Catalysis Materials and Technology, College of Chemistry, Chongqing Normal University, Chongqing 401331, China
b.
Beijing Key Laboratory for Science and Application of Functional Molecular and Crystalline Materials, Department of Chemistry and Chemical Engineering, School of Chemistry and Biological Engineering, University of Science and Technology Beijing, Beijing 100083, China
c.
Key Laboratory of Macrocyclic and Supramolecular Chemistry of Guizhou Province, School of Chemistry and Chemical Engineering, Guizhou University, Guiyang 550025, China

xlliu@cqnu.edu.cn

panhouhe@ustb.edu.cn

xliu@cqnu.edu.cn

jianzhuang@ustb.edu.cn

Received Date: 1 June 2025
Revised Date: 15 October 2025
Accepted Date: 26 October 2025
Available Online: 27 October 2025

Figures(4)

Hydrogen peroxide (H₂O₂), as a green and mild oxidant, exhibits unique application advantages in several fields, including catalytic systems for organic synthesis and environmental pollutant degradation. In recent years, semiconductor-based photocatalytic strategies for H₂O₂ production have attracted extensive attention due to their sustainable characteristics, which utilize H₂O/O₂ as primary reactants to achieve solar-driven chemical energy conversion. Covalent organic frameworks (COFs), with their stable crystalline porous structures, highly ordered π-conjugated systems, modular designability, and ultra-large specific surface areas, provide an ideal platform for photocatalytic H₂O₂ synthesis. Hybridizing COFs with other functional materials has emerged as an effective strategy to address challenges commonly faced by single-component COFs systems, such as low light utilization efficiency, insufficient redox capability, and rapid recombination of photogenerated charge carriers. This review summarizes research progress in COFs-based heterojunctions for photocatalytic H₂O₂ synthesis, beginning with a concise introduction to the photosynthesis mechanism of H₂O₂ and fundamental principles of common heterojunctions in the field, followed by a focused review of reported COFs-based heterojunctions. In addition, the various in-situ applications of H₂O₂ in the context of photosynthesis by COFs-based heterojunctions were discussed, including sterilization, organic pollutants degradation, biomedical applications and organic synthesis. Then concluding with an overview of current challenges and future prospects in this emerging research area. This work aims to promote practical applications of COFs in green energy sectors while providing insights for developing efficient photocatalysts to advance photocatalytic H₂O₂ production.
- Covalent organic frameworks,
- Heterojunction,
- Photocatalysis,
- Hydrogen peroxide,
- Structural engineering,
- In-situ application
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沈阳化工大学材料科学与工程学院沈阳 110142