Citation: Bin Wang, Zichuan Cheng, Fengshuo Xi, Shaoyuan Li, Jijun Lu, Xiuhua Chen, Wenhui Ma. Recent advances in interfacial engineering of lithium battery anodes by atomic layer deposition technology[J]. Chinese Chemical Letters, ;2026, 37(8): 111973. doi: 10.1016/j.cclet.2025.111973 shu

Recent advances in interfacial engineering of lithium battery anodes by atomic layer deposition technology

Bin Wang ^a ,
Zichuan Cheng ^a ,
Fengshuo Xi ^{a, *,} ,
Shaoyuan Li ^{a, *,} ,
Jijun Lu ^a ,
Xiuhua Chen ^b ,
Wenhui Ma ^{a, b, *,}

a.
School of Metallurgical and Energy Engineering/State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 650093, China
b.
School of Engineering/School of Materials Science and Engineering, Yunnan University, Kunming 650091, China

fengshuoxi@126.com

lsy415808550@163.com

mawenhui@ynu.edu.cn

Received Date: 11 August 2025
Revised Date: 12 October 2025
Accepted Date: 15 October 2025
Available Online: 15 October 2025

Figures(13)

Lithium batteries have an exceptional energy density, efficiency, and long service lives, but their anodes show poor interfacial stability. This review summarizes recent advances in the use of atomic layer deposition (ALD) for interfacial modification of lithium battery anodes. It focuses on challenges, including the poor rate performance of intercalation-type anodes, the volume expansion and low initial Coulombic efficiency (ICE) of alloy-type anodes, and dendrite growth and solid-electrolyte interphase (SEI) instability in lithium-metal anodes. Based on this, the multifunctional roles of ALD-derived nanoscale passivation layers in regulating interfacial reactions, suppressing parasitic processes, and enhancing structural integrity are discussed. By evaluating the ability of ALD to improve the cycling lifespan, rate capability, and capacity retention, its application potential for fabricating high-energy-density storage systems is analyzed. This work provides theoretical principles and engineering pathways for the rational design of advanced anode materials.
- Atomic layer deposition,
- Interfacial engineering,
- Lithium battery,
- Anode materials,
- High energy density
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沈阳化工大学材料科学与工程学院沈阳 110142