Citation: Yuheng Wen, Zeyu Wang, Jingli Li, Chengyao Xue, Haobo Wang, Xingrui Li, Hao Zhang, Yang Lu, Yu Zhang, Qing Hou, Wenliang Song. Current advances in heterogeneous catalysts based on hypercrosslinked polymers for transesterification in biodiesel production: A comprehensive review[J]. Chinese Chemical Letters, ;2026, 37(5): 111960. doi: 10.1016/j.cclet.2025.111960 shu

Current advances in heterogeneous catalysts based on hypercrosslinked polymers for transesterification in biodiesel production: A comprehensive review

Yuheng Wen ^a ,
Zeyu Wang ^a ,
Jingli Li ^a ,
Chengyao Xue ^a ,
Haobo Wang ^a ,
Xingrui Li ^a ,
Hao Zhang ^a ,
Yang Lu ^b ,
Yu Zhang ^{c, *,} ,
Qing Hou ^{d, *,} ,
Wenliang Song ^{a, *,}

a.
School of Materials and Chemistry, University of Shanghai for Science and Technology, Shanghai 200093, China
b.
Fuzhou LBE Pharma Tech. Co., Ltd., Fuzhou 350000, China
c.
School of Pharmacy, Shanghai University of Medicine & Health Sciences, Shanghai 201318, China
d.
School of Artificial Intelligence Science and Technology, University of Shanghai for Science and Technology, Shanghai 200093, China

zhangy_21@sumhs.edu.cn

qinghou@usst.edu.cn

wenliang@usst.edu.cn

Received Date: 21 July 2025
Revised Date: 11 October 2025
Accepted Date: 13 October 2025
Available Online: 15 October 2025

Figures(5)

The growing global demand for sustainable energy makes biodiesel an important renewable alternative to alleviate the energy crisis and reduce greenhouse gas emissions. Therefore, there is an urgent need to develop efficient, environmentally friendly and economically viable biodiesel production methods. Hypercrosslinked polymers (HCPs), as aromatic porous organic polymers, are solid frameworks that can be used as heterogeneous catalyst, and they are a promising platform for biodiesel catalytic conversion due to their low cost, highly accessible active site, tunable catalytic site types. In addition, innovative green synthesis strategies make environmentally begin production of HCPs possible. In recent years, HCPs has developed rapidly in the field of biomass catalysis. Unfortunately, to the best of our knowledge, there are no publications focusing on the green synthesis and application of HCPs-based materials for biodiesel production. This review provides an update on the synthesis and utilisation of green and efficient HCPs for catalytic biodiesel production. Initially, the green routes for HCPs synthesis are described, followed by a comprehensive summary of the various approaches to biodiesel production. The primary focus is on the utilisation of HCPs as carriers of active sites in the catalytic conversion of biodiesel, with particular emphasis on catalyst design, morphology control, and intelligent management in terms of application extension. Ultimately, thought-provoking recommendations are proposed to utilize improved green HCPs in combination with advanced production processes to achieve more efficient and sustainable development.
- Hypercrosslinked polymers,
- Green synthesis,
- Catalyst design,
- Highly accessible active site,
- Biodiesel production
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