Citation: Dongfan Li, Jinlong Lv, Jian-Cang Wang, Jiaxiang Liu, Huizhe Niu, Lu Yang, Hao Luo, Du Lv, Lichun Niu, Zemin He, Zongcheng Miao. Interface challenges of solid-state electrolytes/lithium metal anode: From origin analysis, failure mechanism to interface optimization strategies[J]. Chinese Chemical Letters, ;2026, 37(3): 111905. doi: 10.1016/j.cclet.2025.111905 shu

Interface challenges of solid-state electrolytes/lithium metal anode: From origin analysis, failure mechanism to interface optimization strategies

Dongfan Li ^a ,
Jinlong Lv ^a ,
Jian-Cang Wang ^b ,
Jiaxiang Liu ^a ,
Huizhe Niu ^a ,
Lu Yang ^a ,
Hao Luo ^a ,
Du Lv ^a ,
Lichun Niu ^a ,
Zemin He ^{a, *,} ,
Zongcheng Miao ^{c, *,}

a.
Shaanxi Key Laboratory of Liquid Crystal Polymer Intelligent Display, Key Laboratory of Liquid Crystal Polymers based Flexible Display Technology in National Petroleum and Chemical Industry, Technological Institute of Materials & Energy Science (TIMES), Xijing University, Xi'an 710123, China
b.
School of Materials Science and Engineering, Northeastern University, Shenyang 110819, China
c.
School of Artificial Intelligence, Optics and ElectroNics (iOPEN), Northwestern Polytechnical University, Xi'an 710072, China

zeminhe315@126.com

miaozongcheng@nwpu.edu.cn

Received Date: 29 June 2025
Revised Date: 22 September 2025
Accepted Date: 27 September 2025
Available Online: 29 September 2025

Figures(10)

The advent of all-solid-state lithium metal batteries (ASSLMBs) holds promise for overcoming the safety hazards and energy density limitations faced by traditional lithium-ion batteries, thereby advancing the industrialization of next-generation energy storage technologies with high safety and specific energy. However, during practical application, three core challenges persist at the interface between the solid-state electrolytes (SSEs) and the lithium metal anode (LMA): Poor physical contact, interfacial side reactions, and growth of lithium dendrites. These interfacial issues constrain the overall performance of ASSLMBs and impede the commercialization process of this battery system. This review begins by examining the underlying mechanisms responsible for the interfacial problems between SSEs and LMA. Building on this foundation, optimization strategies and recent research progress are systematically introduced, classified according to the interfacial components: SSE-side optimizations, interface engineering, and LMA-side treatments. Finally, future research directions, strategies, and optimization schemes addressing the interfacial challenges between SSEs and LMA are prospected. This analysis aims to facilitate critical breakthroughs in the stability, cycling lifespan, and energy density of ASSLMBs, promoting their transition from laboratory innovation to commercial application.
- All-solid-state lithium metal batteries,
- Solid-state electrolytes,
- Lithium metal anode,
- Interfacial issues,
- Optimization strategies
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沈阳化工大学材料科学与工程学院沈阳 110142