Citation: Ruixuan Chang, Jiachen Zhang, Yawen Tang, Hanjun Sun. Progress in activating lattice oxygen-mediated mechanism in spinel oxides[J]. Chinese Chemical Letters, ;2026, 37(11): 111890. doi: 10.1016/j.cclet.2025.111890 shu

Progress in activating lattice oxygen-mediated mechanism in spinel oxides

Ruixuan Chang ^a ,
Jiachen Zhang ^{a, b} ,
Yawen Tang ^{a, *,} ,
Hanjun Sun ^{a, *,}

a.
School of Chemistry and Materials Science, Jiangsu Key Laboratory of New Power Batteries, Jiangsu Collaborative Innovation Center of Biomedical Functional Materials, Nanjing Normal University, Nanjing 210023, China
b.
School of Chemistry and Chemical Engineering, Southeast University, Nanjing 211189, China

tangyawen@njnu.edu.cn

hanjun.sun@njnu.edu.cn

Received Date: 4 May 2025
Revised Date: 9 August 2025
Accepted Date: 24 September 2025
Available Online: 24 September 2025

Figures(9)

Oxygen evolution reaction (OER) is a pivotal key-reaction in energy technologies, facing kinetic challenges due to multi-step electron transfer. Spinel oxides (AB₂O₄) emerge as promising OER catalysts owing to their dual-cation coordination, enabling electronic structure tailoring. However, their intrinsic configuration favors the adsorbate evolution mechanism (AEM) with a theoretical limitation due to scaling relationships between *OOH and *O intermediates. To overcome the limitation, implementation of the lattice oxygen-mediated mechanism (LOM) becomes imperative. Compared with the AEM, the LOM enables direct O—O coupling to circumvent the inherent scaling relationship limitations, thus arousing widespread attention from researchers. Herein, we firstly systematically investigate the activation prerequisites for transformation from the AEM to the LOM in spinel oxides. Subsequently, rational design strategies to tailor LOM-dominant spinel oxide catalysts are comprehensively summarized. Finally, critical challenges in commercialization are subsequently addressed, outlining a roadmap for advancing these high-performance materials toward industrial energy conversion applications.
- Oxygen evolution reaction,
- Spinel oxide,
- Reaction mechanism,
- LOM pathway,
- Site-selective doping,
- Defect engineering,
- Geometric conversion
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沈阳化工大学材料科学与工程学院沈阳 110142