Citation: Limin Jin, Jie Xu, Huayue Zhu, Chunjuan Li, Zhengfeng Hu, Qi Wang. Recent progress on the (photo)electrocatalytic molecular oxygen activation in reactive oxygen species generation for environmental remediation[J]. Chinese Chemical Letters, ;2026, 37(9): 111865. doi: 10.1016/j.cclet.2025.111865 shu

Recent progress on the (photo)electrocatalytic molecular oxygen activation in reactive oxygen species generation for environmental remediation

Limin Jin ^a ,
Jie Xu ^c ,
Huayue Zhu ^b ,
Chunjuan Li ^{a, *,} ,
Zhengfeng Hu ^{d, *,} ,
Qi Wang ^{a, *,}

a.
Zhejiang Key Laboratory of Solid Waste Pollution Control and Resource Utilization, School of Environmental Science and Engineering, Zhejiang Gongshang University, Hangzhou 310012, China
b.
Institute of Environmental Engineering Technology, Taizhou University, Taizhou 318000, China
c.
Hangzhou Iron & Steel Group Co., LTD, Hangzhou 310022, China
d.
Ecological and Environmental Science and Research Institute of Zhejiang Province, Hangzhou 310007, China

lichunjuan@zjgsu.edu.cn

huzhengfeng2003@163.com

wangqi8327@zjgsu.edu.cn

Received Date: 29 April 2025
Revised Date: 7 August 2025
Accepted Date: 20 September 2025
Available Online: 21 September 2025

Figures(5)

Molecular oxygen (O₂) activation offers a sustainable pathway for environmental remediation by generating reactive oxygen species (ROS), yet challenges in efficiency, stability, and scalability hinder its practical application. This review systematically explores recent advances in integrated (photo)electrocatalytic systems, where synergistic coupling of photonic and electrical energy inputs overcomes spin-forbidden barriers in molecular O₂ activation. Emphasis is placed on nanoscale catalyst engineering, including alloy, carbon-based materials, and single-atom catalysts, to precisely regulate ROS generation via electronic structure design and targeted electron transfer. Parallel innovations in reactor design, such as flow-by and flow-through (photo)electrodes, are analyzed for their role in enhancing mass transport, increasing ROS yields, and ensuring operational durability. Integrating fundamental insights with system engineering, the review provides a roadmap for advancing energy-efficient (photo)electrocatalytic platforms, highlighting their transformative potential in ROS-mediated environmental technologies.
- Molecular oxygen,
- Reactive oxygen species,
- (Photo)electrocatalyst,
- (Photo)electrocatalytic reactor,
- Environmental remediation
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沈阳化工大学材料科学与工程学院沈阳 110142