Citation: Feng Zhao, Hongyu Ding, Ting Sun, Chao Shen, Zu-Li Wang, Wei Wei, Dong Yi. Visible-light-promoted multi-component carbene transfer reactions of diazo compounds via ring-opening of cyclic ethers[J]. Chinese Chemical Letters, ;2026, 37(2): 111834. doi: 10.1016/j.cclet.2025.111834 shu

Visible-light-promoted multi-component carbene transfer reactions of diazo compounds via ring-opening of cyclic ethers

Feng Zhao ^{a, 1} ,
Hongyu Ding ^{b, c, 1} ,
Ting Sun ^a ,
Chao Shen ^{b, *,} ,
Zu-Li Wang ^e ,
Wei Wei ^{c, *,} ,
Dong Yi ^{d, *,}

a.
School of Chemistry and Materials Science, Guizhou Integrated Research Center of Polymer Electromagnetic Materials, Key Laboratory of Functional Organic Molecule, Guizhou Education University, Guiyang 550018, China
b.
Zhejiang Collaborative Innovation Center for Full-Process Monitoring and Green Governance of Emerging Contaminants, College of Biology and Environmental Engineering, Zhejiang Shuren University, Hangzhou 310015, China
c.
School of Chemistry and Chemical Engineering, Qufu Normal University, Qufu 273165, China
d.
Green Pharmaceutical Technology Key Laboratory of Luzhou City, School of Pharmacy, Southwest Medical University, Luzhou 646000, China
e.
College of Chemical Engineering, Nanjing Forestry University, Nanjing 210037, China

shenchaozju@zjsru.edu.cn

weiweiqfnu@163.com

yidong@swmu.edu.cn

Received Date: 19 July 2025
Revised Date: 1 September 2025
Accepted Date: 11 September 2025
Available Online: 13 September 2025

Figures(37)

Carbenes as one of the most important class of intermediates have been widely utilized in various organic synthetic transformations. Carbene insertion-initiated ring-opening reactions of cyclic ethers offer a valuable strategy for constructing new carbon-oxygen bonds. In comparison with traditional thermal or metal-mediated carbene transfer reactions, visible-light-promoted multi-component reaction strategy provides a mild and eco-friendly approach to access densely functionalized molecules. Recently, visible-light-induced multi-component carbene transfer reactions of diazo compounds have been rapidly developed and attracted a great deal of research interest of chemists owing to their advantages of simple operation, mild condition, high atom economy and rich structural diversity. This paper summarizes the recent research progress on the visible-light-promoted multi-component carbene transfer reactions of diazo compounds via ring-opening of cyclic ethers with various nucleophiles. The reaction patterns of different nucleophiles and their corresponding mechanism are described in this review. The future research direction and challenges in this area are also discussed.
- Visible-light,
- Multi-component reaction,
- Carbene insertion,
- Diazo compounds,
- Ring-opening reaction
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