Citation: Kang Zhang, Jin Zhao, Pengcheng Su, Mingkun Wang, Kexin Wan, Hongwei Tang, Dai-Huo Liu, Jingyu Sun, Yihui Li. Molecular engineering strategies of ammonium vanadates for advanced zinc-ion storage[J]. Chinese Chemical Letters, ;2026, 37(7): 111831. doi: 10.1016/j.cclet.2025.111831 shu

Molecular engineering strategies of ammonium vanadates for advanced zinc-ion storage

Kang Zhang ^a ,
Jin Zhao ^{b, *,} ,
Pengcheng Su ^a ,
Mingkun Wang ^a ,
Kexin Wan ^a ,
Hongwei Tang ^a ,
Dai-Huo Liu ^a ,
Jingyu Sun ^{b, *,} ,
Yihui Li ^{a, *,}

a.
Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals, Key Laboratory of Green Chemical Media and Reactions, Ministry of Education, School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang 453007, China
b.
College of Energy, Soochow Institute for Energy and Materials InnovationS (SIEMIS), Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu Province, Soochow University, Suzhou 215006, China

jzhaoenergy@stu.suda.edu.cn

sunjy86@suda.edu.cn

liyihui@htu.edu.cn

Received Date: 30 June 2025
Revised Date: 8 September 2025
Accepted Date: 11 September 2025
Available Online: 11 September 2025

Figures(12)

Aqueous zinc-ion batteries (ZIBs) have gained tremendous interests by virtue of their intrinsic safety, low cost and favorable theoretical capacities. As the promising candidates of cathode materials of ZIBs, ammonium vanadates (NVO) have captured widespread attentions owing to their tunable chemical properties and enhanced structural stabilities owing to the existence of NH₄⁺ in the [VO]_n layers. However, the pristine NVO fails to meet the expectations due to the strong interlayer electrostatic repulsion and comparatively sluggish transfer kinetics, which necessitates the exploration of appropriate modification strategies to fully dig its potential. Herein, this review systematically summarizes five core molecular engineering strategies, intercalation, defect, interfacial, doping, and structural engineering strategies, and their significances in modulating structural and electrochemical properties of NVO are elaborately discussed. Moreover, the perspectives on the future developments and potential energy-related applications of NVO are presented. This review is anticipated to deepen the researchers' understandings of the potentials of molecular engineering strategies on improving zinc-ion storage capabilities of cathode materials, and further promote the practicality of NVO in ZIBs.
- Molecular engineering strategies,
- Ammonium vanadates,
- Zinc-ion storage,
- Structural modulation,
- Enhanced transfer kinetics
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沈阳化工大学材料科学与工程学院沈阳 110142