Citation: Qi Li, Minqiao Liang, Huifen Zhuang, Zhengyang Chen, Yuxiang Jiang, Xiaofei Chen, Yifa Chen, Ya-Qian Lan. Underscoring the polyimide-linkage in covalent organic frameworks and related applications[J]. Chinese Chemical Letters, ;2026, 37(2): 111593. doi: 10.1016/j.cclet.2025.111593 shu

Underscoring the polyimide-linkage in covalent organic frameworks and related applications

Qi Li ^{a, 1} ,
Minqiao Liang ^{a, 1} ,
Huifen Zhuang ^a ,
Zhengyang Chen ^a ,
Yuxiang Jiang ^a ,
Xiaofei Chen ^{b, *,} ,
Yifa Chen ^{a, *,} ,
Ya-Qian Lan ^{a, *,}

a.
School of Chemistry, South China Normal University, Guangzhou 510006, China
b.
Key Laboratory for Special Functional Materials of Ministry of Education National & Local Joint Engineering Research Center for High-Efficiency Display and Lighting Technology, School of Nanoscience and Materials Engineering, Henan University, Kaifeng 475004, China

Author Bio: Qi Li received his M.S. degree (2019) from Nanjing Normal University and his Engineering Ph.D. degree (2024) from Southeast University under the supervision of Prof. Zeng-Mei Wang and in collaboration with Prof. Ya-Qian Lan. Since 2024, he has been conducting postdoctoral research at South China Normal University with Prof. Yifa Chen. His current research focuses on the syntheses of COF-based crystalline porous materials and their applications in energy storage and conversion
Minqiao Liang was born in 2004 in Guangdong, China. She is now a chemistry undergraduate at South China Normal University under the supervision of Prof. Ya-Qian Lan and Prof. Yifa Chen. Her research interest focuses on the syntheses of crystalline porous materials (COF-based composites) and their applications in energy storage and conversion

Xiaofei Chen received her Ph.D. degree in polymer chemistry and physics from Jilin University under the supervision of Prof. Lixin Wu in 2021. Currently, she works at the Key Laboratory for Special Functional Materials of the Ministry of Education, Henan University, China. Her current research focuses on the syntheses of polyoxometalate based supramolecular complexes as well as COF and their applications in photocatalysis and photothermal catalysis
Yifa Chen received his B.S. degree from School of Chemistry, Beijing Institute of Technology. He subsequently obtained his Ph.D. degree from School of Chemistry and Chemical Engineering, Beijing Institute of Technology under the supervision of Prof. Bo Wang. In 2022, he joined South China Normal University (SCNU, China) as a professor of chemistry. His research interest focuses on the fabrication of porous crystalline material based devices like membranes, foams and fibers that can be applicable in photo-/electro-catalysis, energy storage or environment treatment
Ya-Qian Lan received his B.S. and Ph.D. degrees (2009) from Northeast Normal University under the supervision of Prof. Zhong-Min Su. In 2010, he joined the National Institute of Advanced Industrial Science and Technology (AIST, Japan) as a JSPS postdoctoral fellow. In 2012, he became a professor of chemistry at Nanjing Normal University (NNU, China). In 2021, he joined South China Normal University (SCNU, China) as a professor of chemistry. His current research interest focuses on the synthesis of new crystalline materials and catalytic research related to clean energy applications

chenxf22@henu.edu.cn

chenyf927821@163.com

yqlan@m.scnu.edu.cn

Received Date: 11 May 2025
Revised Date: 8 July 2025
Accepted Date: 16 July 2025
Available Online: 18 July 2025

Figures(11)

Polyimide-linkage covalent organic frameworks (PI-COFs), as a subclass of the COFs material family, featuring the unique combination of excellent thermal stability of polyimide, tunable pore sizes, as well as high crystallinity and surface area of COFs, are expected to be a novel type of promising crystalline porous material with potential applications in adsorption and separation, catalysis, chemical sensing, and energy storage. Therefore, it is increasingly important to summarize polyimide-linkage in COFs and related applications and provide in-depth insight to accelerate future development. In this review, we offer a comprehensive overview of recent advancements in PI-COFs, emphasizing their synthesis methods, design principles and applications. Finally, our brief outlooks on the current challenges and future developments of PI-COFs are provided. Overall, this review aims to guide the recent and future development of PI-COFs.
- Covalent organic frameworks,
- Polyimide-linkage,
- Heteroatomic sites,
- Chemical stability,
- Thermal stability
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沈阳化工大学材料科学与工程学院沈阳 110142