Citation: Huijie Zhou, Mutawara Mahmood Baig, Shunyu Gu, Wenjiang Zou, Jing Zhang, Fei Dou, Jiang Xu, Lvzhou Li, Yizhou Zhang, Huan Pang, Jianning Ding. Design, synthesis, and optimization of MXene- and MOF-based materials for 3D printed energy storage devices and beyond[J]. Chinese Chemical Letters, ;2026, 37(9): 111489. doi: 10.1016/j.cclet.2025.111489 shu

Design, synthesis, and optimization of MXene- and MOF-based materials for 3D printed energy storage devices and beyond

Huijie Zhou ^{a, b} ,
Mutawara Mahmood Baig ^{b, c} ,
Shunyu Gu ^b ,
Wenjiang Zou ^a ,
Jing Zhang ^a ,
Fei Dou ^b ,
Jiang Xu ^a ,
Lvzhou Li ^a ,
Yizhou Zhang ^{c, *,} ,
Huan Pang ^{a, b, *,} ,
Jianning Ding ^{a, *,}

a.
Institute of Technology for Carbon Neutralization, Yangzhou University, Yangzhou 225127, China
b.
School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou 225009, China
c.
Institute of Advanced Materials and Flexible Electronics (IAMFE), School of Chemistry and Materials Science, Nanjing University of Information Science and Technology, Nanjing 210044, China

Author Bio:

Prof. Yi-Zhou Zhang received his Bachelor's degree from Nanjing University, after which he obtained a PhD from Nanjing University of Posts & Telecommunications. He is now a professor of Materials Science and Engineering at Nanjing University of Information Science and Technology (NUIST) and head of the institute of Advanced Materials and Flexible electronics in NUIST. Prof. Zhang mainly works on functional materials for printed and flexible energy storage and electronics. Due to his contributions to this field, he has been recognized as a Highly Cited Researcher by Clarivate in 2023 and 2024
Huan Pang is a distinguished professor at Yangzhou University. He received his Ph.D. degree from Nanjing University in 2011. He is now a Young Changjiang Scholar of the Ministry of Education in China, and a senior member of the Chinese Chemical Society. He is the managing editor of EnergyChem, editorial board member of FlatChem and Rare Metals, and youth editorial board member of Nano Research and eScience among other distinguished academic journals. He has won "Best Editor Award 2021″ for his professional excellence and outstanding contribution to Nano Research. His research area mainly focuses on MOFs related materials
Jianning Ding received his Ph.D. degree from Tsinghua University in 2001. Now, he is doing research at Yangzhou University as a professor. Prof. Jianning Ding's research interests focus on flexible mechatronics, new energy technology, and equipment functional devices, including solar cells, flexible sensors, soft robotics, and so on

yizhou.zhang@nuist.edu.cn

panghuan@yzu.edu.cn

dingjn@yzu.edu.cn

Received Date: 23 January 2025
Revised Date: 17 June 2025
Accepted Date: 18 June 2025
Available Online: 24 June 2025

Figures(17)

MXene and metal-organic frame (MOFs) are emerging as transformative materials in the field of energy storage and conversion. While MXene excel in conductivity, tunable surface chemistry, and flexibility, MOFs bring complementary benefits with their tunable porosity and structural versatility, enabling the design of hybrid systems with enhanced functionalities. However, challenges such as material stability, structural integrity, and ink formulation must be addressed to fully integrate these materials into 3D printing technologies. This review elucidates cutting-edge material design frameworks for MXene- and MOF-integrated 3D-printed architectures, emphasizing their transformative roles in advancing energy storage/conversion systems. We provide a systematic evaluation of additive manufacturing compatibility and multidisciplinary optimization strategies spanning ink rheology, hierarchical structure engineering, and interfacial electrochemistry to enhance device performance metrics. Additionally, by analyzing the key advantages and limitations of MXene- and MOF-based materials, we examine their role in overcoming current challenges in electrochemical energy storage devices. Finally, we provide insights into future prospects, presenting a roadmap for integrating MXene and MOFs into scalable 3D printing technologies, which will enable breakthroughs in sustainable and high-performance energy devices.
- MXene,
- MOF,
- Mixed inks,
- 3D printing,
- Energy storage devices
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