Citation: Fengchen Wang, Yujia Xiang, Yuqi Zhang, Xin Zhou, Jing Zhang, Chuanshu He, Heng Zhang, Zhaokun Xiong, Peng Zhou, Hongyu Zhou, Yang Liu, Bo Lai. A comprehensive review on oxygen vacancies modified catalysts: Synthesis, characterization, and crucial role in catalytic ozonation[J]. Chinese Chemical Letters, ;2026, 37(2): 111315. doi: 10.1016/j.cclet.2025.111315 shu

A comprehensive review on oxygen vacancies modified catalysts: Synthesis, characterization, and crucial role in catalytic ozonation

Fengchen Wang ^a ,
Yujia Xiang ^a ,
Yuqi Zhang ^a ,
Xin Zhou ^a ,
Jing Zhang ^{a, b} ,
Chuanshu He ^a ,
Heng Zhang ^{a, b} ,
Zhaokun Xiong ^{a, b} ,
Peng Zhou ^{a, b} ,
Hongyu Zhou ^c ,
Yang Liu ^{a, b, d, *,} ,
Bo Lai ^{a, b, d, *,}

a.
State Key Laboratory of Hydraulics and Mountain River Engineering, College of Architecture and Environment, Sichuan University, Chengdu 610065, China
b.
Sino-German Centre for Water and Health Research, Sichuan University, Chengdu 610065, China
c.
School of Chemical Engineering, The University of Adelaide, Adelaide, SA 5005, Australia
d.
Water Safety and Water Pollution Control Engineering Technology Research Center in Sichuan Province, Haitian Water Group, Chengdu 610041, China

liuyang_scu@scu.edu.cn

laibo@scu.edu.cn

Received Date: 15 October 2024
Revised Date: 6 March 2025
Accepted Date: 14 May 2025
Available Online: 14 May 2025

Figures(6)

Among various advanced oxidation processes (AOPs), heterogeneous catalytic ozonation has garnered extensive attention in wastewater treatment owing to its broad pH range applicability and the elimination of the need for additional energy input. Enhancing catalyst activity by introducing oxygen vacancies has been used extensively in heterogeneous catalytic ozonation. This paper reviews prevalent methods for the construction and characterization of oxygen vacancies. Based on a thorough examination of existing research, the role of oxygen vacancies is categorized according to their primary mechanisms of action in heterogeneous catalytic ozonation. For example, modulation of the catalyst electronic structure to enhance electron transfer; participation in the reaction as an active site to generate radicals and non-radicals; and exposure of more metal sites to enhance the reaction. Lastly, the paper delineates the limitations and future research directions concerning the role of oxygen vacancies in catalytic ozonation. This review addresses the gap in existing literature concerning the role of oxygen vacancies in catalytic ozone systems, establishes a comprehensive theoretical framework to aid in the design of efficient ozone catalysts, and delves into the functionality of oxygen vacancies in heterogeneous catalytic ozone reactions.
- Catalytic ozonation,
- Bulk defects,
- Surface defects,
- Oxygen vacancies,
- Degradation mechanism,
- Synthesis and characterization
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沈阳化工大学材料科学与工程学院沈阳 110142