Citation: Jiahao Li, Bin Pan, Anruo Mao, Likui Wang, Dawei Wang. Construction of effective and recyclable non-noble metal coordination polymers and their multiple applications in water[J]. Chinese Chemical Letters, ;2026, 37(1): 111165. doi: 10.1016/j.cclet.2025.111165 shu

Construction of effective and recyclable non-noble metal coordination polymers and their multiple applications in water

Jiahao Li ^a ,
Bin Pan ^b ,
Anruo Mao ^c ,
Likui Wang ^a ,
Dawei Wang ^{a, d, *,}

a.
Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering, Jiangnan University, Wuxi 214122, China
b.
Shandong Engineering Research Center of Green and High-value Marine Fine Chemical, Weifang University of Science and Technology, Shouguang 262700, China
c.
Department of Chemistry, University of Manchester, Oxford Road, Manchester M13 9PL, United Kingdom
d.
Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, Shanghai 200032, China

wangdw@jiangnan.edu.cn

wangdw@sioc.ac.cn

Received Date: 18 August 2024
Revised Date: 19 March 2025
Accepted Date: 1 April 2025
Available Online: 2 April 2025

Figures(15)

Acceptorless dehydrogenative coupling of pyridinemethanol with ketones is one of the most reliable methodologies to access functionalized 1,8-naphthyridine derivatives. However, it is challenging to develop environmentally friendly catalytic systems, especially in constructing efficient and recyclable catalysts under water or solvent-free conditions. Here, we designed two novel coordination polymers Cd–CPs and Fe–CPs to investigate their catalytic performance in water. Gratifyingly, it was observed that Cd-CPs as a multifunctional catalyst was successfully applied to establish a universal pathway for direct fabrication of 1,8-naphthyridine derivatives under water conditions, while it was effective for the synthesis of 1,3,5-triazines through acceptorless dehydrogenative coupling strategies. The features of broad substrate, high atom efficiency, and good catalyst reusability highlight the feasibility of this transformation. In additional, we demonstrated the spindle-like structures Fe-P, derived from the Fe–CPs via phosphorylation, which can be used as an efficient electrocatalyst for oxygen evolution reaction with good stability. This work provides two highly efficient non-noble metal catalysts for functionalized 1,8-naphthyridine derivatives production and oxygen evolution reaction, and opens a new avenue to further fabricate diverse metal catalysts with high catalytic performance in water.
- Acceptorless dehydrogenative coupling,
- 1,8-Naphthyridine derivatives,
- Coordination polymers,
- Non-noble metal catalyst
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沈阳化工大学材料科学与工程学院沈阳 110142