Citation: Yaxuan Fu, Xiaozhi Jiang, Chenyang Shi, Long Chen, Zhendong Yang, Mengran Wang, Bo Hong, Faping Zhong, Yanqing Lai. The role of flame-retardant electrolytes in lithium-ion batteries: Custom design for improved battery-level safety[J]. Chinese Chemical Letters, ;2026, 37(4): 110972. doi: 10.1016/j.cclet.2025.110972 shu

The role of flame-retardant electrolytes in lithium-ion batteries: Custom design for improved battery-level safety

Yaxuan Fu ^a ,
Xiaozhi Jiang ^a ,
Chenyang Shi ^a ,
Long Chen ^a ,
Zhendong Yang ^a ,
Mengran Wang ^{a, b, c, d, *,} ,
Bo Hong ^{a, b, c, d, *,} ,
Faping Zhong ^d ,
Yanqing Lai ^{a, b, c, d, e}

a.
School of Metallurgy and Environment, Central South University, Changsha 410083, China
b.
Engineering Research Centre of Advanced Battery Materials, The Ministry of Education, Changsha 410083, China
c.
National Energy Metal Resources and New Materials Key Laboratory, Changsha 410083, China
d.
National Engineering Research Center of Advanced Energy Storage Materials, Changsha 410083, China
e.
Hunan Province Key Laboratory of Nonferrous Value-Added Metallurgy, Central South University, Changsha 410083, China

mengranwang93@163.com

bop_hong@csu.edu.cn

Received Date: 2 November 2024
Revised Date: 11 February 2025
Accepted Date: 18 February 2025
Available Online: 18 February 2025

Figures(7)

With the increasing demand for high-energy-density lithium ion batteries, it has become increasingly imperative to address the safety concerns associated with batteries. At present, the design of flame-retardant electrolytes has been widely studied. However, most strategies lack the discussion of battery-level safety, and have only conducted primary safety tests such as ignition. In this situation, it is necessary to analyze the intrinsic link between flame-retardant electrolytes and battery safety. This paper elucidates the role of flame-retardant electrolytes in the thermal runaway process of batteries and proposes a strategy to enhance the safety of batteries from the aspect of electrolytes. Then the thermal, electrochemical and interfacial stability characteristics of different flame-retardant electrolytes are analyzed in detail based on their structures, and the basic principles for the design of their solvent structures are pointed out to enhance electrochemical performance. Furthermore, a prospective summary of safety characterization at the material and battery level is presented, aiming to build a comprehensive battery safety characterization system. This review provides insights into the design of flame-retardant electrolytes for high safety batteries.
- Flame-retardant electrolytes,
- Battery-level safety,
- Safety characterization,
- Thermal runaway,
- Lithium-ion battery
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沈阳化工大学材料科学与工程学院沈阳 110142