Citation: Linlin Gan, Xuan Peng, Wenchao Zhai, Cheng Zhang, Xinyu Duan, Ke Deng, Wei Li, Qingdao Zeng. Regulatory effects of coronene and pyridine on the self-assembly structure of tetracarboxylic acid derivative formed by dimeric building blocks[J]. Chinese Chemical Letters, ;2026, 37(3): 110667. doi: 10.1016/j.cclet.2024.110667 shu

Regulatory effects of coronene and pyridine on the self-assembly structure of tetracarboxylic acid derivative formed by dimeric building blocks

Linlin Gan ^{a, 1} ,
Xuan Peng ^{c, 1} ,
Wenchao Zhai ^c ,
Cheng Zhang ^d ,
Xinyu Duan ^c ,
Ke Deng ^{a, *,} ,
Wei Li ^{c, *,} ,
Qingdao Zeng ^{a, b, *,}

a.
CAS key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology (NCNST), Beijing 100190, China
b.
Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
c.
School of Science, Nanchang Institute of Technology, Nanchang 330099, China
d.
School of Materials Science and Engineering, South China University of Technology, Guangzhou 510641, China

kdeng@nanoctr.cn

liweidting@nit.edu.cn

zengqd@nanoctr.cn

Received Date: 25 September 2024
Revised Date: 7 November 2024
Accepted Date: 21 November 2024
Available Online: 23 November 2024

Figures(6)

The regulation of guest molecules on the self-assembly system of tetracarboxylic acid derivative (H₄BDETP) at the liquid/solid interface was studied by scanning tunneling microscopy (STM) and density functional theory (DFT) calculations. Coronene (COR) guest molecules induced H₄BDETP to transform from linear assembly structure to diversified nanoporous structures in which COR could be captured. And the regulation of pyridine guest molecules (DPE, BPYB, TYPY) on the mono-component assembly structure of H₄BDETP was achieved by forming O–H···N hydrogen bonds with H₄BDETP. The introduction of both COR and pyridine derivatives could destroy the hydrogen-bonded dimers of H₄BDETP, and new O–H···O hydrogen bonds were formed between H₄BDETP molecules. In addition, H₄BDETP/pyridine co-assembly structures depended on the central bridging units and the number of pyridine groups in pyridine derivatives. Furthermore, H₄BDETP/TYPY structure underwent structural transformation induced by COR and multi-component assembly structures with thermodynamic stability were constructed.
- Regulation,
- Co-assembly,
- Hydrogen bond,
- Pyridine,
- STM
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