Citation: Ming Yang, Lin-Bo Liu, Shuo Liu, Yan Li, Biao Ouyang, Xian-Zhu Fu, Jing-Li Luo, Yifei Sun, Subiao Liu. Electrosynthesizing high-value fuels from CO₂ in solid oxide electrolysis cells: Fundamentals, advances, and perspectives[J]. Chinese Chemical Letters, ;2025, 36(12): 110603. doi: 10.1016/j.cclet.2024.110603 shu

Electrosynthesizing high-value fuels from CO₂ in solid oxide electrolysis cells: Fundamentals, advances, and perspectives

Ming Yang ^a ,
Lin-Bo Liu ^a ,
Shuo Liu ^a ,
Yan Li ^a ,
Biao Ouyang ^a ,
Xian-Zhu Fu ^b ,
Jing-Li Luo ^{b, c} ,
Yifei Sun ^{d, *,} ,
Subiao Liu ^{a, *,}

a.
School of Minerals Processing and Bioengineering, Central South University, Changsha 410083, China
b.
College of Materials Science and Engineering, Shenzhen University, Shenzhen 518060, China
c.
Department of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta T6G 1H9, Canada
d.
College of Energy, Xiamen University, Xiamen 361005, China

yfsun@xmu.edu.cn

subiao@csu.edu.cn

Received Date: 11 September 2024
Revised Date: 11 October 2024
Accepted Date: 1 November 2024
Available Online: 2 November 2024

Figures(10)

The rising level of CO₂ concentration in the atmosphere poses major threats to the global climate and environment. Various technologies have been developed to mitigate its negative effects through non-conversion and conversion routes. Particularly, solid oxide electrolysis cells (SOECs), as a promising technology with the highest energy efficiency, have garnered considerable attention for their effectiveness to electrochemically convert CO₂ into high-value fuels. However, the insufficient catalytic activity, poor long-term stability, and high costs have significantly hindered the industrial-scale application of SOECs. To this end, substantial efforts, with an emphasis on the smart design of targeting electrode materials for specific applications have been devoted to advancing the electrosynthesis of high-value fuels from CO₂ in various SOECs, but there still lacks a critical and comprehensive review in-depth discussing the fundamentals, and summarizing the latest advances in various applications and electrode materials for electrochemically converting CO₂ to high-value fuels in SOECs. This review thus aims to fill this gap by focusing on the fundamentals (i.e., SOEC working principles, thermodynamics, kinetics and representative evaluation parameters), specific applications (i.e., pure CO₂ electrolysis, CO₂-H₂O co-electrolysis, fuel-assisted CO₂ conversion), and material selection criteria (i.e., cathodic materials for CO₂ conversion, and anodic materials for fuel-assisted CO₂ conversion). In addition, the challenges that this technology is currently facing, and our perspectives on electrochemical CO₂ conversion in SOECs are proposed to guide the smart design of high-performance electrocatalysts and future industrial-scale application of SOECs for electrosynthesizing high-value fuels from CO₂.
- Solid oxide electrolysis cell,
- Perovskite oxide,
- CO₂ electrolysis,
- Co-electrolysis,
- Alkane dehydrogenation,
- Syngas production
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Electrosynthesizing high-value fuels from CO2 in solid oxide electrolysis cells: Fundamentals, advances, and perspectives

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通讯作者: 陈斌, bchen63@163.com

Electrosynthesizing high-value fuels from CO₂ in solid oxide electrolysis cells: Fundamentals, advances, and perspectives