Citation: Jinjiang Wu, Zhenhua Zhu, Jinkui Tang. Recent advancements of photo-responsive lanthanide single-molecule magnets[J]. Chinese Chemical Letters, ;2025, 36(12): 110577. doi: 10.1016/j.cclet.2024.110577 shu

Recent advancements of photo-responsive lanthanide single-molecule magnets

Jinjiang Wu ^{a, b, c} ,
Zhenhua Zhu ^b ,
Jinkui Tang ^{b, c, *,}

a.
School of Chemistry and Chemical Engineering, North University of China, Taiyuan 030051, China
b.
State Key Laboratory of Rare Earth Resource Utilization, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China
c.
School of Applied Chemistry and Engineering, University of Science and Technology of China, Hefei 230026, China

tang@ciac.ac.cn

Received Date: 20 September 2024
Revised Date: 18 October 2024
Accepted Date: 22 October 2024
Available Online: 24 October 2024

Figures(7)

The dynamic regulation of single-molecule magnet (SMM) behavior remains challenging but extremely critical to practical applications. Efficient manipulation of magnetization of complexes via external stimulus, like solvent, pressure, electric potential or light may further extend the scope of applications for these magnetic molecules. Among these, light is highly desirable because it can provide high-contrast, sensitive and remote control of magnetic behavior at relatively high spatial and temporal resolution. Lanthanide (Ln) complexes represent a distinctive platform for constructing photo-responsive SMMs owing to their extreme sensitivity to subtle change of crystal field (CF) environment. Despite the numerous potential benefits and unique advantages outlined above, light control of magnetism of Ln-SMMs still faces several challenges. This review briefly summarizes recent advancements of photo-responsive Ln-SMMs with photochromic characteristic, highlighting the significance of photoinduced structural changes or electronic distribution alterations to modulate the magnetic properties, which may throw light on the future improvements of photo-responsive molecular materials.
- Single-molecule magnets,
- Lanthanide,
- Dynamic regulation,
- Photo-responsive,
- Photochromism
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