Citation: Qiang-Qiang Jia, Jia-Qi Luo, Zhi-Yu Xue, Jing-Song Tang, Wen-Qiang Qiu, Chang-Feng Wang, Zhi-Xu Zhang, Hai-Feng Lu, Yi Zhang, Da-Wei Fu. Enhanced output power density of PVDF/LM composite for piezoelectric sensor[J]. Chinese Chemical Letters, ;2025, 36(11): 110471. doi: 10.1016/j.cclet.2024.110471 shu

Enhanced output power density of PVDF/LM composite for piezoelectric sensor

Qiang-Qiang Jia ^{a, 1} ,
Jia-Qi Luo ^{a, 1} ,
Zhi-Yu Xue ^a ,
Jing-Song Tang ^a ,
Wen-Qiang Qiu ^a ,
Chang-Feng Wang ^a ,
Zhi-Xu Zhang ^a ,
Hai-Feng Lu ^{a, *,} ,
Yi Zhang ^{a, *,} ,
Da-Wei Fu ^{a, b, *,}

a.
Institute for Science and Applications of Molecular Ferroelectrics, Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Zhejiang Normal University, Jinhua 321004, China
b.
Ordered Matter Science Research Center, Jiangsu Key Laboratory for Science and Applications of Molecular Ferroelectrics, Southeast University, Nanjing 211189, China

luhaifeng@zjnu.edu.cn

yizhang1980@seu.edu.cn

dawei@seu.edu.cn

Received Date: 9 July 2024
Revised Date: 3 September 2024
Accepted Date: 17 September 2024
Available Online: 18 September 2024

Figures(5)

Poly(vinylidene fluoride) (PVDF) based piezoelectric materials have received tremendous scientific attention for many decades. However, the high output power density remains a significant challenge and an area of intense interest. Herein, we present a piezoelectric sensor with high output power density by incorporating liquid metal (LM) microdroplets into PVDF piezoelectric substrate. Remarkably, the LM/PVDF composite showed the β-phase content above 90% and the output power density is enhanced to 353 µW/cm², nearly 1000 times higher than that of pure PVDF materials and significantly surpassing other PVDF-based composite materials. These exceptional performances are attributed to two key factors: The formation of a liquid-solid/electric-dielectric interface between the LM and PVDF, and the incorporation of the LM's outstanding charge transfer capability. This work might present an effective strategy for advancing the utilization of PVDF-based piezoelectric materials in compelling applications within the realm of intelligent wearable electronics.
- PVDF,
- Liquid metal,
- Piezoelectric,
- Ferroelectric,
- Flexible self-powered sensing
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