Citation: Jiaming Li, Na Xu, Yafei Zhang, Hongjun Dong, Chunmei Li. Research progress of heterogeneous photocatalyst for H₂O₂ production: A mini review[J]. Chinese Chemical Letters, ;2025, 36(11): 110470. doi: 10.1016/j.cclet.2024.110470 shu

Research progress of heterogeneous photocatalyst for H₂O₂ production: A mini review

Jiaming Li ^{a, b} ,
Na Xu ^{a, *,} ,
Yafei Zhang ^{c, *,} ,
Hongjun Dong ^b ,
Chunmei Li ^{b, *,}

a.
College of Chemistry, Jilin Normal University, Siping 136000, China
b.
Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, China
c.
Biofuels Institute, School of the Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China

xuna@jlnu.edu.cn

yf-zhang@ujs.edu.cn

lcmdhj@ujs.edu.cn

Received Date: 24 July 2024
Revised Date: 12 September 2024
Accepted Date: 17 September 2024
Available Online: 19 September 2024

Figures(15)

H₂O₂ is an excellent green oxidant with important applications in many fields. The conventional anthraquinone process for synthesizing H₂O₂ is usually accompanied by high economic costs and stringent process requirements. The photocatalytic production of H₂O₂ via heterojunction semiconductors has proven to overcome these limitations, which is a promising alternative to the conventional anthraquinone process. In this review, we provide a comprehensive summary of the semiconductor heterojunction materials that have been attempted to be used in the photocatalytic generation of H₂O₂ in recent years. Firstly, a brief description of the photoreaction mechanisms of different types of heterojunctions in the photocatalytic process is presented, focusing on the generation pathways and competing reactions for the photoproduction of H₂O₂. Then, the types of heterojunctions applied for photoproduction of H₂O₂ are comprehensively summarized. Among them, the four most widely used types of heterojunctions, including type-Ⅱ heterojunctions, Z-scheme systems, S-scheme systems, and Schottky heterojunctions, and their current applications in the reaction of photoproduction of H₂O₂ are highlighted. By comparing the differences in the internal electric fields of different types of heterojunctions, different charge transfer pathways of various types of heterojunctions in the photoproduction of H₂O₂ are distinguished. Furthermore, the great potential of other types of heterojunctions, such as p-n heterojunctions, in photocatalysis is further outlined. Finally, the challenges as well as opportunities for the development of novel heterostructural photocatalysts for H₂O₂ production are outlined. We sincerely hope this minireview can attract more attention from scientific research workers in the field of photocatalytic H₂O₂ generation, making them valuable for environmental remediation and industrial applications in the future.
- Heterojunction,
- Photocatalysis,
- H₂O₂ production,
- Design strategy,
- Reaction mechanism
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Research progress of heterogeneous photocatalyst for H2O2 production: A mini review

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Research progress of heterogeneous photocatalyst for H₂O₂ production: A mini review