Citation: Liyong Ding, Zhenhua Pan, Qian Wang. 2D photocatalysts for hydrogen peroxide synthesis[J]. Chinese Chemical Letters, ;2024, 35(12): 110125. doi: 10.1016/j.cclet.2024.110125 shu

2D photocatalysts for hydrogen peroxide synthesis

Liyong Ding ^{a, b} ,
Zhenhua Pan ^d ,
Qian Wang ^{a, c, *,}

a.
Graduate School of Engineering, Nagoya University, Furo-cho, Chikusa-ku, Nagoya 464-8603, Japan
b.
College of Chemical and Material Engineering, Quzhou University, Quzhou 324000, China
c.
Institute for Advanced Research, Nagoya University, Furo-cho, Chikusa-ku, Nagoya 464-8601, Japan
d.
Department of Applied Chemistry, Graduate School of Engineering, University of Hyogo, Himeji, Hyogo 671-2280, Japan

wang.qian@material.nagoya-u.ac.jp

Received Date: 8 April 2024
Revised Date: 7 June 2024
Accepted Date: 13 June 2024
Available Online: 18 June 2024

Figures(7)

Photocatalytic hydrogen peroxide (H₂O₂) synthesis, driven by solar energy, offers a sustainable and cleaner alternative for producing green H₂O₂ from water and oxygen. 2D photocatalysts have emerged as powerful materials for this purpose due to their unique physiochemical properties such as a flexible planar structure and large surface area. This review provides a comprehensive overview of the latest advances in 2D photocatalytic materials employed in H₂O₂ synthesis, including metal oxides, metal chalcogenides, bismuth-based materials, graphitic carbon nitrides (g-C₃N₄), metal−organic frameworks (MOFs), and covalent organic frameworks (COFs). Beginning with an extensive introduction to possible reaction routes for photocatalytic H₂O₂ synthesis, we summarize the common methods for H₂O₂ detection, crucial for obtaining reliable results in H₂O₂ studies. Additionally, we highlight molecular-level modification strategies for 2D photocatalysts, such as surface modification, ion doping, defect engineering, and heterojunction construction, which promote high-efficiency solar-to-chemical conversion for sustainable H₂O₂ photosynthesis. Furthermore, we discuss key issues and provide perspective outlooks for the efficient and sustainable generation of H₂O₂ in scale-up industrial production. This review offers in-depth insights into different reaction pathways of H₂O₂ synthesis and provides design principles for 2D photocatalysts to enhance H₂O₂ production, guiding the development of efficient photocatalysts for H₂O₂ synthesis.
- Photocatalysis,
- Hydrogen peroxide production,
- 2D photocatalysts,
- Oxygen reduction reaction,
- Water oxidation reaction
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