Citation: Ziyou Zhang, Te Ji, Hongliang Dong, Zhiqiang Chen, Zhi Su. Effect of coordination restriction on pressure-induced fluorescence evolution[J]. Chinese Chemical Letters, ;2024, 35(12): 109542. doi: 10.1016/j.cclet.2024.109542 shu

Effect of coordination restriction on pressure-induced fluorescence evolution

Ziyou Zhang ^{a, b} ,
Te Ji ^c ,
Hongliang Dong ^b ,
Zhiqiang Chen ^{b, *,} ,
Zhi Su ^{a, *,}

a.
Jiangsu Collaborative Innovation Center of Biomedical Functional Materials, College of Chemistry and Materials Science, Nanjing Normal University, Nanjing 210046, China
b.
Center for High Pressure Science and Technology Advanced Research, Shanghai 201203, China
c.
Shanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201204, China

chenzq@hpstar.ac.cn

zhisu@njnu.edu.cn

Received Date: 22 December 2023
Revised Date: 12 January 2024
Accepted Date: 17 January 2024
Available Online: 24 January 2024

Figures(4)

The usage of flexible ligands in constructing MOF materials (FL-MOFs) has been widely studied due to its numerous advantages, including the structural diversity, polynuclear MOFs, transmitting magnetic exchanges, enantioselective separation, asymmetric catalysis, etc. However, the field still faces challenges in deeply understanding the effect of ligand configuration on the properties of these materials. Here, we employ a flexible aggregation-induced emission ligand (4,4′-((1E, 1′E)-anthracene-9,10-diylbis(ethene-2,1-diyl))dibenzoic acid) with great mechanical stability to construct FL-MOFs to lock the ligand configuration to explore the pressure-induced evolution of the ligand with coordination restriction, involving changes in fluorescence and intermolecular interaction. In-situ high-pressure fluorescence, Raman, and FT-IR experiments have revealed that the intermolecular interaction of AIE-Mn-MOF with configuration restriction increased more rapidly than that of free AIE-L. This discovery offers valuable insights for synthesizing MOF materials with exceptional mechanical stability and significantly advances our understanding of the impact of coordination restriction in FL-MOFs on their response to external stimuli.
- Coordination chemistry,
- High-pressure chemistry,
- FL-MOFs,
- High-pressure photoluminescent,
- Coordination restriction
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