Citation: Kexin Yuan, Yulei Liu, Haoran Feng, Yi Liu, Jun Cheng, Beiyang Luo, Qinglian Wu, Xinyu Zhang, Ying Wang, Xian Bao, Wanqian Guo, Jun Ma. Unlocking the potential of thin-film composite reverse osmosis membrane performance: Insights from mass transfer modeling[J]. Chinese Chemical Letters, ;2024, 35(5): 109022. doi: 10.1016/j.cclet.2023.109022 shu

Unlocking the potential of thin-film composite reverse osmosis membrane performance: Insights from mass transfer modeling

Kexin Yuan ^a ,
Yulei Liu ^a ,
Haoran Feng ^a ,
Yi Liu ^a ,
Jun Cheng ^a ,
Beiyang Luo ^a ,
Qinglian Wu ^{a, b} ,
Xinyu Zhang ^c ,
Ying Wang ^d ,
Xian Bao ^{a, *,} ,
Wanqian Guo ^a ,
Jun Ma ^a

a.
State Key Laboratory of Urban Water Resource and Environment, School of Environment, Harbin Institute of Technology, Harbin 150090, China
b.
College of Architecture and Environment, Sichuan University, Chengdu 610065, China
c.
School of Municipal and Environmental Engineering, Shandong Jianzhu University, Ji'nan 250101, China
d.
College of Water Conservancy and Hydropower Engineering, Sichuan Agricultural University, Yaan 625014, China

baoxian24@163.com

Received Date: 18 July 2023
Revised Date: 19 August 2023
Accepted Date: 29 August 2023
Available Online: 2 September 2023

Figures(4)

Thin-film composite (TFC) reverse osmosis (RO) membranes have attracted considerable attention in water treatment and desalination processes due to their specific separation advantages. Nevertheless, the trade-off effect between water flux and salt rejection poses huge challenges to further improvement in TFC RO membrane performance. Numerous research works have been dedicated to optimizing membrane fabrication and modification for addressing this issue. In the meantime, several reviews summarized these approaches. However, the existing reviews seldom analyzed these methods from a theoretical perspective and thus failed to offer effective optimization directions for the RO process from the root cause. In this review, we first propose a mass transfer model to facilitate a better understanding of the entire process of how water and solute permeate through RO membranes in detail, namely the migration process outside the membrane, the dissolution process on the membrane surface, and the diffusion process within the membrane. Thereafter, the water and salt mass transfer behaviors obtained from model deduction are comprehensively analyzed to provide potential guidelines for alleviating the trade-off effect between water flux and salt rejection in the RO process. Finally, inspired by the theoretical analysis and the accurate identification of existing bottlenecks, several promising strategies for both regulating RO membranes and optimizing operational conditions are proposed to further exploit the potential of RO membrane performance. This review is expected to guide the development of high-performance RO membranes from a mass transfer theory standpoint.
- Reverse osmosis,
- Mass transfer model,
- Trade-off effect,
- Membrane performance,
- Optimization strategies
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沈阳化工大学材料科学与工程学院沈阳 110142