Citation: Qingyun Li, Ziqing Hu, Xiaofan Ji. AIE interfacial supramolecular polymers[J]. Chinese Chemical Letters, ;2024, 35(1): 108741. doi: 10.1016/j.cclet.2023.108741 shu

AIE interfacial supramolecular polymers

Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan 430074, China

xiaofanji@hust.edu.cn

Received Date: 20 April 2023
Revised Date: 24 June 2023
Accepted Date: 26 June 2023
Available Online: 27 June 2023

Figures(6)

High monomer concentration is a requisite for engendering the aggregation-induced emssion (AIE) phenomenon as well as the formation of supramolecular polymers. Therefore, this is supposed to ensure the generation of AIE supramolecular polymers, wherein the monomer soluability takes effect. Nevertheless, parts of supramolecular monomers are considered as poessessing different soluability towards the same sovlent, through which the polymerzation process is thus hard to proceed. Interfacial polymerzation gets over the soluabilty restriction, providing a facile method for propelling the reaction of thesemonomers. Herein, we had prepared M1 containing tetraphenylethene (TPE) functionalized with two terpyridine derivatives, then making M1 dissolving in CHCl₃ to give solutions. Cu²⁺ solutions were fabricated through dissolving CuCl₂ into H₂O. Towards mixing those solutions, AIE interfacial supramolecular polymers (AIEISPs) displaying green fluorescence were generated at the interface of two phases on the basis of metal-coordination between terpyridine and Cu²⁺. These AIEISPs were certificated to possess the stimuli-responsiveness, for which the excessive addition of tetrabutylammonium hydroxide would cause the structure destruction owing to the stronger bonding ability with Cu²⁺ than that of terpyridine. These fabricated AIEISPs had provided a new avenue to prepare AIE supramolecular polymers.
- Aggregation-induced emission,
- Interfaces,
- Metal-coordination interactions,
- Supramolecular polymers,
- Stimuli-responsiveness
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