Citation: Yuan Zhang, Shenghao Gong, A.R. Mahammed Shaheer, Rong Cao, Tianfu Liu. Plasmon-enhanced photocatalytic oxidative coupling of amines in the air using a delicate Ag nanowire@NH₂-UiO-66 core-shell nanostructures[J]. Chinese Chemical Letters, ;2024, 35(4): 108587. doi: 10.1016/j.cclet.2023.108587 shu

Plasmon-enhanced photocatalytic oxidative coupling of amines in the air using a delicate Ag nanowire@NH₂-UiO-66 core-shell nanostructures

Yuan Zhang ^{a, b, c, 1} ,
Shenghao Gong ^{a, b, c, 1} ,
A.R. Mahammed Shaheer ^{a, c} ,
Rong Cao ^{a, b, c, *,} ,
Tianfu Liu ^{a, b, c, *,}

a.
Fujian Science Technology Innovation Laboratory for Optoelectronic Information of China, Fuzhou 350108, China
b.
College of Chemistry and Materials Science, Fujian Normal University, Fuzhou 350007, China
c.
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China

rcao@fjirsm.ac.cn

tfliu@fjirsm.ac.cn

Received Date: 12 April 2023
Revised Date: 4 May 2023
Accepted Date: 17 May 2023
Available Online: 20 May 2023

Figures(5)

MOF-based core-shell structures with high surface area, abundant active sites, and broad absorption bands are viable alternatives to traditional single-component photocatalysts. In this report, we describe the design and construction of delicate Ag nanowires@NH₂-UiO-66 with a core-shell structure for use as photocatalysts in imine synthesis under light. The optimized composites exhibited 80% imine production, which was higher than both MOF and Ag NWs. The significant improvement in photocatalytic activity under light may be attributed to the plasmonic effect of silver nanowires and their core-shell structure, which promotes the separation of electron-hole pairs. Moreover, the photocatalytic activity of the core-shell nanostructure may provide valuable insight into the design and construction of MOF-based composite photocatalysts for oxidative coupling of amines.
- Metal-organic frameworks,
- Plasmonic silver nanowires,
- Photocatalyst,
- Core-shell nanostructure,
- Oxidative coupling of amines
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Plasmon-enhanced photocatalytic oxidative coupling of amines in the air using a delicate Ag nanowire@NH2-UiO-66 core-shell nanostructures

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通讯作者: 陈斌, bchen63@163.com

Plasmon-enhanced photocatalytic oxidative coupling of amines in the air using a delicate Ag nanowire@NH₂-UiO-66 core-shell nanostructures