Citation: Sajid Mahmood, Haiyan Wang, Fang Chen, Yijun Zhong, Yong Hu. Recent progress and prospects of electrolytes for electrocatalytic nitrogen reduction toward ammonia[J]. Chinese Chemical Letters, ;2024, 35(4): 108550. doi: 10.1016/j.cclet.2023.108550 shu

Recent progress and prospects of electrolytes for electrocatalytic nitrogen reduction toward ammonia

Sajid Mahmood ^{a, b} ,
Haiyan Wang ^{a, *,} ,
Fang Chen ^c ,
Yijun Zhong ^a ,
Yong Hu ^{a, c, *,}

a.
Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Department of Chemistry, Zhejiang Normal University, Jinhua 321004, China
b.
The Center for Applied Mathematics and Bioinformatics (CAMB), Gulf University for Science and Technology, Mishref 32093, Kuwait
c.
Hangzhou Institute of Advanced Studies, Zhejiang Normal University, Hangzhou 311231, China

chemwhy@zjnu.edu.cn

yonghu@zjnu.edu.cn

Received Date: 1 April 2023
Revised Date: 13 April 2023
Accepted Date: 8 May 2023
Available Online: 14 May 2023

Figures(18)

Electrochemical nitrogen reduction reaction (ENRR) provides a promising strategy to achieve sustainable synthesis of ammonia. However, despite great efforts devoted to this research field, the problems such as low energy efficiency and weak selectivity still impede its practical implementation. Most of the research to date has been concentrated on creating sophisticated electrocatalysts, and adequate knowledge of electrolytes is still lacking. Herein, the recent progress in electrolytes for ENRR, including alkaline, neutral, acidic, water-in-salt, organic, ionic liquid, and mixed water-organic electrolytes, is thoroughly reviewed to obtain an in-depth understanding of their effects on electrocatalytic performance. Recently developed representative electrocatalysts in various types of electrolytes are also introduced, and future research priorities of different electrolytes are proposed to develop new and efficient ENRR systems.
- Electrocatalytic nitrogen reduction,
- Ammonia,
- Electrolytes,
- Production rate,
- Faradaic efficiency
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沈阳化工大学材料科学与工程学院沈阳 110142