Citation: Jinrong Huo, Kai Zhang, Haocong Wei, Ling Fu, Chenxu Zhao, Chaozheng He, Xincheng Hu. A review on hydrogen production from ammonia borane: Experimental and theoretical studies[J]. Chinese Chemical Letters, ;2023, 34(12): 108280. doi: 10.1016/j.cclet.2023.108280 shu

A review on hydrogen production from ammonia borane: Experimental and theoretical studies

Jinrong Huo ^{a, c} ,
Kai Zhang ^{a, c} ,
Haocong Wei ^{a, c} ,
Ling Fu ^e ,
Chenxu Zhao ^{c, d} ,
Chaozheng He ^{c, d, *,} ,
Xincheng Hu ^{b, *,}

a.
School of Sciences, Xi'an Technological University, Xi'an 710021, China
b.
Henan Engineering Center of New Energy Battery Materials, College of Chemistry and Chemical Engineering, Shangqiu Normal University, Shangqiu 476000, China
c.
School of Materials Science and Chemical Engineering, Institute of Environmental and Energy Catalysis, Xi'an Technological University, Xi'an 710021, China
d.
Shaanxi Key Laboratory of Optoelectronic Functional Materials and Devices, School of Materials Science and Chemical Engineering, Xi'an Technological University, Xi'an 710021, China
e.
College of Resources and Environmental Engineering, Tianshui Normal University, Tianshui 741001, China

hecz2019@xatu.edu.cn

huxincheng2019@163.com

Received Date: 20 December 2022
Revised Date: 18 February 2023
Accepted Date: 28 February 2023
Available Online: 3 March 2023

Figures(19)

Ammonia borane (NH₃BH₃, AB) is an ideal raw material of hydrogen production with higher hydrogen storage capacity. In this paper, the catalytic processes of AB dehydrogenation were described from different ways, including thermal dehydrogenation, hydrolysis, methanolysis, photocatalysis and photo-piezoelectric synergy catalysis with experimental research and theoretical calculations. Catalyst models include bulk materials, two-dimensional materials, nanocluster particles and single/diatomic structures. Among them, the proportion of H₂ released is different, and the reaction conditions are also different, which are suitable for different application scenarios. Through this review, we could have a preliminary comprehensive understanding of AB dehydrogenation reaction.
- Ammonia borane,
- Hydrogen production,
- Dehydrogenation catalyst,
- Hydrolysis,
- Methanolysis,
- Photo-piezoelectric synergy
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