Citation: Ruonan Guo, Ying Chen, Ying Yang, Jiangwei Shang, Xiuwen Cheng. Efficient degradation of sulfacetamide by CoFe PBAs and PBA@PVDF composite membrane activating peroxymonosulfate[J]. Chinese Chemical Letters, ;2023, 34(5): 107837. doi: 10.1016/j.cclet.2022.107837 shu

Efficient degradation of sulfacetamide by CoFe PBAs and PBA@PVDF composite membrane activating peroxymonosulfate

Ruonan Guo ^a ,
Ying Chen ^a ,
Ying Yang ^a ,
Jiangwei Shang ^{a, b} ,
Xiuwen Cheng ^{a, b, *,}

a.
Key Laboratory for Environmental Pollution Prediction and Control, Gansu Province, College of Earth and Environmental Sciences, Lanzhou University, Lanzhou 730000, China
b.
Key Laboratory of Pollutant Chemistry and Environmental Treatment, College of Chemistry and Environmental Science, Yili Normal University, Yining 835000, China

chengxw@lzu.edu.cn

Received Date: 14 January 2022
Revised Date: 23 August 2022
Accepted Date: 19 September 2022
Available Online: 23 September 2022

Figures(4)

More and more antibiotics that are difficult to biodegrade have been detected in water environments threatening ecosystems and human health. Therefore, it is urgent to develop efficient water treatment methods to degrade antibiotics. In this work, Co-Fe Prussian blue analogues (PBAs) with different molar ratios were synthesized for peroxymonosulfate (PMS) activation to degrade sulfacetamide (SAM, 10 mg/L). By increasing Co molar ratio, the PMS activation capability and electrochemical properties of PBAs were enhanced. Due to its excellent reactivity (degradation efficiency of 84.2% and mineralization efficiency of 52.79%), cost benefit (electrical energy per order, 0.01019 kWh/L) and lower metal leaching ([Co] = 0.259 mg/L, [Fe] = 0.128 mg/L), PBA-1, the as-prepared catalyst with a molar ratio of cobalt to iron of 1:1, was selected for further study. The radical scavenging experiments and an electron paramagnetic resonance (EPR) trapping experiments were performed and revealed that PBA-1 addition was required to produced ^•OH and SO₄^•− from PMS activation. Accordingly, we proposed a PMS activation mechanism and SAM decomposition pathways for PBA-1/PMS reaction system. Besides, a PBA-1@polyvinylidene fluoride (PVDF) catalytic membrane was further prepared to expand the application potential of PBA nanoparticles. The PBA-1@PVDF catalytic membrane was highly effective and exhibited a great reusability; thus, it could be considered for applications in actual water treatment processes.
- Prussian blue analogues,
- Peroxymonosulfate,
- Sulfacetamide,
- Composite membrane
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