Citation: Ruding Zhang, Huixin Chen, Hongjun Yue. Room-temperature synthesis of layered open framework cathode for sodium-ion batteries[J]. Chinese Chemical Letters, ;2023, 34(5): 107580. doi: 10.1016/j.cclet.2022.06.003 shu

Room-temperature synthesis of layered open framework cathode for sodium-ion batteries

Ruding Zhang ^{a, b} ,
Huixin Chen ^{a, b} ,
Hongjun Yue ^{a, b, *,}

a.
CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China
b.
Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institutes, Chinese Academy of Sciences, Xiamen 361021, China

hjyue@fjirsm.ac.cn

Received Date: 5 May 2022
Revised Date: 21 May 2022
Accepted Date: 1 June 2022
Available Online: 3 June 2022

Figures(4)

The synthesis of active electrode materials at room temperature is one of the effective strategies to reduce the fabrication cost of sodium ion batteries (SIBs). Herein, a layered material (Na₂[(VO)₂(HPO4)₂C₂O₄]·2H₂O, abbreviated as NVPC followingly) with open-framework structures has been successfully prepared at room temperature under ambient conditions and is evaluated as a cathode for SIBs. It is revealed that NVPC cathode can deliver a maximum reversible capacity of ca. 70 mAh/g at 10 mA/g, and exhibit superior rate capability and cycling performance: at 50 mA/g, maximum reversible capacity ca. 50 mAh/g with capacity retention of 88.4% over 250 cycles corresponds to only 0.046% capacity decay per cycle; at 100 mA/g, a maximum reversible capacity of 35 mAh/g with capacity retention of 60.9% over 500 cycles. This study demonstrates a practical example of a low-cost synthesis of the cathode materials for SIBs. At the same time, the systematic electrochemical research results also show promising prospects for long lifespan low-cost SIBs.
- Room temperature solution synthesis,
- Open framework structure,
- Cathode materials,
- Sodium-ion batteries,
- Full cell
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