Citation: Xianjin Shi, Leo N.Y. Cao, Meijuan Chen, Yu Huang. Recent progress on two-dimensional materials confining single atoms for CO₂ photoreduction[J]. Chinese Chemical Letters, ;2022, 33(12): 5023-5029. doi: 10.1016/j.cclet.2022.01.066 shu

Recent progress on two-dimensional materials confining single atoms for CO₂ photoreduction

Xianjin Shi ^{a, b, c} ,
Leo N.Y. Cao ^{d, e} ,
Meijuan Chen ^f ,
Yu Huang ^{a, b, *,}

a.
Key Laboratory of Aerosol Chemistry and Physics, State Key Laboratory of Loess and Quaternary Geology (SKLLQG), Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China
b.
Center of Excellence in Quaternary Science and Global Change, Chinese Academy of Sciences, Xi'an 710061, China
c.
University of Chinese Academy of Sciences, Beijing 100049, China
d.
CAS Center for Excellence in Nanoscience, Beijing Key Laboratory of Micro-nano Energy and Sensor, Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of Sciences, Beijing 101400, China
e.
School of Nanoscience and Technology, University of Chinese Academy of Sciences, Beijing 100049, China
f.
School of Human Settlements and Civil Engineering, Xi'an Jiaotong University, Xi'an 710049, China

huangyu@ieecas.cn

Received Date: 17 November 2021
Revised Date: 11 December 2021
Accepted Date: 25 January 2022
Available Online: 1 February 2022

Figures(3)

Photoreduction of CO₂ into value-added products offers a promising approach to overcome both climate change and energy crisis. However, low conversion efficiency, poor product selectivity, and unclear mechanism limit the further advancement of CO₂ photoreduction. The development of two-dimensional (2D) materials and construction of single atom sites are two frontier research fields in catalysis. Combining the advantages of 2D materials and single atom sites is expected to make a breakthrough in CO₂ photoreduction. In this review, we summarized the design and application, proposed challenges and opportunities, and laid a foundation for further research and application of 2D materials confining single atoms (SACs@2D) for CO₂ photoreduction.
- CO₂ reduction,
- Photocatalyst,
- Single atom,
- 2D materials,
- g-C₃N₄
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Recent progress on two-dimensional materials confining single atoms for CO2 photoreduction

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通讯作者: 陈斌, bchen63@163.com

Recent progress on two-dimensional materials confining single atoms for CO₂ photoreduction