Citation: Weiwei Wang, Xibao Li, Fang Deng, Jiyou Liu, Xiaoming Gao, Juntong Huang, Jilin Xu, Zhijun Feng, Zhi Chen, Lu Han. Novel organic/inorganic PDI-Urea/BiOBr S-scheme heterojunction for improved photocatalytic antibiotic degradation and H₂O₂ production[J]. Chinese Chemical Letters, ;2022, 33(12): 5200-5207. doi: 10.1016/j.cclet.2022.01.058 shu

Novel organic/inorganic PDI-Urea/BiOBr S-scheme heterojunction for improved photocatalytic antibiotic degradation and H₂O₂ production

Weiwei Wang ^a ,
Xibao Li ^{a, b, *,} ,
Fang Deng ^b ,
Jiyou Liu ^a ,
Xiaoming Gao ^c ,
Juntong Huang ^a ,
Jilin Xu ^a ,
Zhijun Feng ^a ,
Zhi Chen ^a ,
Lu Han ^{d, *,}

a.
School of Materials Science and Engineering, Nanchang Hangkong University, Nanchang 330063, China
b.
Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, Nanchang 330063, China
c.
Department of Chemistry and Chemical Engineering, Shaanxi Key Laboratory of Chemical Reaction Engineering, Yan'an University, Yan'an 716000, China
d.
School of Materials and Metallurgy, University of Science and Technology Liaoning, Anshan 114051, China

lixibao@nchu.edu.cn

hanlu@ustl.edu.cn

Received Date: 20 October 2021
Revised Date: 10 December 2021
Accepted Date: 23 January 2022
Available Online: 31 January 2022

Figures(5)

The matched energy band structure and efficient carrier separation efficiency are the keys to heterogeneous photocatalytic reactions. A novel organic/inorganic step scheme (S-scheme) heterojunction PDI-Urea/BiOBr composite photocatalyst was constructed by simple solvothermal reaction combined with in-situ growth strategy. The composite photocatalyst not only has high chemical stability, but also can generate and accumulate a large number of active species (h⁺, ^•O₂⁻, ^•OH, H₂O₂). PDI-Urea/BiOBr showed higher photocatalytic activity for the degradation of antibiotic such as ofloxacin (OFLO), tetracycline (TC) and the production of H₂O₂ in the spectral range of 400–800 nm. The apparent rate constant of 15% PDI-Urea/BiOBr for photocatalytic degradation of TC (or OFLO) was 2.7 (or 2.5) times that of pure BiOBr and 1.7 (or 1.8) times that of pure PDI-Urea. The H₂O₂ evolution rate of 15% PDI-Urea/BiOBr was 2.5 times that of PDI-Urea and 1.5 times that of BiOBr, respectively. This work has formed a mature S-scheme heterojunction design thought and method, which offers new visions for the development of heterogeneous photocatalysts.
- Photocatalysis,
- Perylene diimide,
- Bismuth bromide oxide,
- S-scheme heterojunction,
- Antibiotic
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沈阳化工大学材料科学与工程学院沈阳 110142

Novel organic/inorganic PDI-Urea/BiOBr S-scheme heterojunction for improved photocatalytic antibiotic degradation and H2O2 production

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通讯作者: 陈斌, bchen63@163.com

Novel organic/inorganic PDI-Urea/BiOBr S-scheme heterojunction for improved photocatalytic antibiotic degradation and H₂O₂ production