Citation: Xiao-Zhong Fan, Meng Liu, Ruiqi Zhang, Yuezhou Zhang, Songcan Wang, Haoxiong Nan, Yunhu Han, Long Kong. An odyssey of lithium metal anode in liquid lithium–sulfur batteries[J]. Chinese Chemical Letters, ;2022, 33(10): 4421-4427. doi: 10.1016/j.cclet.2021.12.064 shu

An odyssey of lithium metal anode in liquid lithium–sulfur batteries

Xiao-Zhong Fan ^a ,
Meng Liu ^a ,
Ruiqi Zhang ^a ,
Yuezhou Zhang ^{a, b} ,
Songcan Wang ^{a, b} ,
Haoxiong Nan ^c ,
Yunhu Han ^{a, *,} ,
Long Kong ^{a, *,}

a.
Frontiers Science Center for Flexible Electronics and Xi'an Institute of Flexible Electronics (IFE), Northwestern Polytechnical University, Xi'an 710129, China
b.
Ningbo Institute of Northwestern Polytechnical University, Ningbo 315103, China
c.
School of Science, Hainan University, Haikou 570228, China

iamyhhan@nwpu.edu.cn

iamlkong@nwpu.edu.cn

Received Date: 16 November 2021
Revised Date: 14 December 2021
Accepted Date: 23 December 2021
Available Online: 29 December 2021

Figures(3)

Lithium–sulfur (Li–S) batteries exhibit outstanding energy density and material sustainability. Enormous effects have been devoted to the sulfur cathode to address redox kinetics and polysulfide intermediates shuttle. Recent attentions are gradually turning to the protection of the lithium metal anodes, since electrochemical performances of Li–S batteries are closely linked to the working efficiency of the anode side, especially in pouch cells that adopt stringent test protocols. This Perspective article summarizes critical issues encountered in the lithium metal anode, and outlines possible solutions to achieve efficient working lithium anode in Li–S batteries. The lithium metal anode in Li–S batteries shares the common failure mechanisms of volume fluctuation, nonuniform lithium flux, electrolyte corrosion and lithium pulverization occurring in lithium metal batteries with oxide cathodes, and also experiences unique polysulfide corrosion and massive lithium accumulation. These issues can be partially addressed by developing three-dimensional scaffold, exerting quasi-solid reaction, tailoring native solid electrolyte interphase (SEI) and designing artificial SEI. The practical evaluation of Li–S batteries highlights the importance of pouch cell platform, which is distinguished from coin-type cells in terms of lean electrolyte-to-sulfur ratio, thin lithium foil, as well as sizable total capacity and current that are loaded on pouch cells. This Perspective underlines the development of practically efficient working lithium metal anode in Li–S batteries.
- Lithium–sulfur batteries,
- Lithium metal anode,
- Electrolytes,
- Solid electrolyte interphase,
- Pouch cell
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沈阳化工大学材料科学与工程学院沈阳 110142