Citation: Yonggang Xue, Liqin Wang, Suixin Liu, Yu Huang, Long Chen, Long Cui, Yan Cheng, Junji Cao. High impact of vehicle and solvent emission on the ambient volatile organic compounds in a major city of northwest China[J]. Chinese Chemical Letters, ;2022, 33(5): 2753-2756. doi: 10.1016/j.cclet.2021.11.013 shu

High impact of vehicle and solvent emission on the ambient volatile organic compounds in a major city of northwest China

Yonggang Xue ^{a, b, c} ,
Liqin Wang ^{a, b, c} ,
Suixin Liu ^{a, b, c} ,
Yu Huang ^{a, b, c, *,} ,
Long Chen ^{a, b, c} ,
Long Cui ^{a, b, c} ,
Yan Cheng ^d ,
Junji Cao ^{a, b, c}

a.
State Key Lab of Loess and Quaternary Geology (SKLLQG), Institute of Earth Environment, Chinese Academy of Sciences (CAS), Xi'an 710061, China
b.
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an 710061, China
c.
Guanzhong Plain Ecological Environment Change and Comprehensive Treatment National Observation and Research Station, Xi'an 710061, China
d.
School of Human Settlements and Civil Engineering, Xi'an Jiaotong University, Xi'an 710049, China

huangyu@ieecas.cn

Received Date: 24 August 2021
Revised Date: 9 October 2021
Accepted Date: 2 November 2021
Available Online: 10 November 2021

Figures(3)

Monitoring of ambient volatile organic compounds (VOCs) was conducted within typical residential-commercial area in the city of Xi'an in northwest China during typical ozone (O₃) episodes, to investigate the major contributors to the characteristic of ambient VOCs and their impact on O₃ production. In the residential-commercial area, diurnal variation of VOCs was highly impacted by vehicle exhaust, fuel evaporation, and local solvent use. Relative higher contributions (up to 60%) of VOCs from solvent use to the ozone formation potential were found. The present findings highlight the urgent need for restrictions on the emission of VOCs from solvent use and non-vehicle-traffic-related sources, such as oil storage.
- VOCs,
- Vehicle exhaust,
- Fuel evaporation,
- Solvent using,
- Northwest China
1. [1]
  P.J. Nowack, N.L. Abraham, P. Braesicke, J.A. Pyle, J. Geophys. Res. Atmos. 123(2018) 4630-4641. doi: 10.1002/2017JD027943
2. [2]
  M. Russell, Science 241(1988) 1275-1276. doi: 10.1126/science.3413490
3. [3]
  Z. Ma, J. Xu, W. Quan, et al., Atmos. Chem. Phys. 16(2016) 3969-3977. doi: 10.5194/acp-16-3969-2016
4. [4]
  T. Wang, X.L. Wei, A.J. Ding, et al., Atmos. Chem. Phys. 9(2009) 6217-6227. doi: 10.5194/acp-9-6217-2009
5. [5]
  R. Dang, H. Liao, Y. Fu, Sci. Total Environ. 754(2021) 142394. doi: 10.1016/j.scitotenv.2020.142394
6. [6]
  K. Li, D.J. Jacob, H. Liao, et al., Proc. Natl. Acad. Sci. U. S. A. 116(2019) 422-427. doi: 10.1073/pnas.1812168116
7. [7]
  X. Lu, L. Zhang, X. Wang, et al., Environ. Sci. Technol. Lett. 7(2020) 240-247. doi: 10.1021/acs.estlett.0c00171
8. [8]
  H. Zhao, K. Chen, Z. Liu, et al., Chemosphere 270(2021) 129441. doi: 10.1016/j.chemosphere.2020.129441
9. [9]
  L.K. Xue, T. Wang, J. Gao, et al., Atmos. Chem. Phys. 14(2014) 13175-13188. doi: 10.5194/acp-14-13175-2014
10. [10]
  Z. Yuan, A.K.H. Lau, M. Shao, et al., J. Geophys. Res. Atmos. 114(2009) D00G15.
11. [11]
  Y. Xue, S.S.H. Ho, Y. Huang, et al., Sci. Rep. 7(2017) 9979. doi: 10.1038/s41598-017-10631-4
12. [12]
  Y. Xue, Y. Huang, S.S.H. Ho, et al., Atmos. Chem. Phys. 20(2020) 5425-5436. doi: 10.5194/acp-20-5425-2020
13. [13]
  L. Hui, T. Ma, Z. Gao, et al., Chemosphere 265(2021) 129072-129072. doi: 10.1016/j.chemosphere.2020.129072
14. [14]
  R.X. Luo, B.S. Liu, D.N. Liang, et al., Huanjing kexue 42(2021) 75-87.
15. [15]
  B. Yuan, M. Shao, S. Lu, B. Wang, Atmos. Environ. 44(2010) 1919-1926. doi: 10.1016/j.atmosenv.2010.02.014
16. [16]
  R. Wu, S. Xie, Environ. Sci. Technol. 51(2017) 2574-2583. doi: 10.1021/acs.est.6b03634
17. [17]
  T. Feng, N.F. Bei, R.J. Huang, et al., Atmos. Chem. Phys. 16(2016) 4323-4342. doi: 10.5194/acp-16-4323-2016
18. [18]
  T. Feng, S. Zhao, X. Zhang, et al., Sci. Total Environ. 745(2020) 140961. doi: 10.1016/j.scitotenv.2020.140961
19. [19]
  M. Shao, S.H. Lu, Y. Liu, et al., J. Geophys. Res. Atmos. 114(2009) D00G06. doi: 10.1029/2008JD010863
20. [20]
  Y. Zou, X. Deng, D. Zhu, et al., Atmos. Chem. Phys. 15(2015) 6625-6636. doi: 10.5194/acp-15-6625-2015
21. [21]
  Y. Huang, Z.H. Ling, S.C. Lee, et al., Atmos. Environ. 122(2015) 809-818. doi: 10.1016/j.atmosenv.2015.09.036
22. [22]
  Y. Liu, L. Kong, X. Liu, et al., Atmos. Pollut. Res. 12(2021) 33-46. doi: 10.1016/j.apr.2021.01.013
23. [23]
  Y. Zhang, L. Xue, W.P.L. Carter, et al., Atmos. Chem. Phys. 21(2021) 11053-11068. doi: 10.5194/acp-21-11053-2021
24. [24]
  Y. Liu, M. Shao, L. Fu, et al., Atmos. Environ. 42(2008) 6247-6260. doi: 10.1016/j.atmosenv.2008.01.070
25. [25]
  A.E. Perring, S.E. Pusede, R.C. Cohen, Chem. Rev. 113(2013) 5848-5870. doi: 10.1021/cr300520x
26. [26]
  R. Atkinson, J. Arey, Chem. Rev. 103(2003) 4605-4638. doi: 10.1021/cr0206420
27. [27]
  K.F. Ho, S.C. Lee, W.K. Ho, et al., Atmos. Chem. Phys. 9(2009) 7491-7504. doi: 10.5194/acp-9-7491-2009
28. [28]
  Y. Zhang, X. Wang, Z. Zhang, et al., Atmos. Environ. 79(2013) 110-118. doi: 10.1016/j.atmosenv.2013.06.029
29. [29]
  B. Li, S.S.H. Ho, Y. Xue, et al., Atmos. Environ. 161(2017) 1-12. doi: 10.1016/j.atmosenv.2017.04.029
30. [30]
  USEPA, EPA Positive Matrix Factorization (PMF) 5.0 Fundamentals and User Guide, Washington DC, U. S. A. 2014.
31. [31]
  W.P.L. Carter, J. Air Waste Manage. 44(1994) 881-899. doi: 10.1080/1073161X.1994.10467290
1. [1]
  YUE Xu , WANG Sheng , GAO Yang , LIU Xu , LI De-yi , WANG Jian-cheng , HAO Bing-yuan , WANG Shu-dong . Thermodynamics analysis on the adsorption behaviors of VOCs on various adsorbents. Journal of Fuel Chemistry and Technology, 2020, 48(6): 752-760.
2. [2]
  Zhang Chao , Li Sihan , Wu Chenliang , Li Xiaoqing , Yan Xinhuan . Preparation and Characterization of Pt@Au/Al₂O₃ Core-Shell Nanoparticles for Toluene Oxidation Reaction. Acta Physico-Chimica Sinica, 2020, 36(8): 1907057-0. doi: 10.3866/PKU.WHXB201907057
3. [3]
  Jun GENG , Quan-li KE , Wen-xi ZHOU , Wu-jian WANG , Shan-hu WANG , Ying ZHOU , Han-feng LU . Research progress in the sulfur resistance of catalytic combustion catalysts. Journal of Fuel Chemistry and Technology, 2022, 50(5): 564-575. doi: 10.1016/S1872-5813(21)60182-2
4. [4]
  Qingjun Yu , Yongchao Feng , Jinghui Wei , Xiaolong Tang , Honghong Yi . Development of Mn-Si-MEL as a bi-functional adsorption-catalytic oxidation material for VOCs elimination. Chinese Chemical Letters, 2022, 33(6): 3087-3090. doi: 10.1016/j.cclet.2021.09.072
5. [5]
  LI Si-Han , LI Xiao-Qing , HU Feng-Teng , ZHANG Chao , YAN Xin-Huan . Catalytic Oxidation of Toluene with Low Loading Bimetallic Au@Pt Core-Shell Catalyst. Chinese Journal of Inorganic Chemistry, 2019, 35(3): 553-562. doi: 10.11862/CJIC.2019.055
6. [6]
  Ying Wu , Yu-Dong Yang , Min Shao , Si-Hua Lu . Missing in total OH reactivity of VOCs from gasoline evaporation. Chinese Chemical Letters, 2015, 26(10): 1246-1248. doi: 10.1016/j.cclet.2015.05.047
7. [7]
  YANG Zheng-Zheng , YANG Yi , ZHAO Ming , NG Mao-Chu , CHEN Yao-Qiang . Enhanced Sulfur Resistance of Pt-Pd/CeO₂-ZrO₂-Al₂O₃ Commercial Diesel Oxidation Catalyst by SiO₂ Surface Cladding. Acta Physico-Chimica Sinica, 2014, 30(6): 1187-1193. doi: 10.3866/PKU.WHXB201404281
8. [8]
  CAO Hong-Yan , WANG Jian-Li , YAN Sheng-Hui , LIU Zhi-Min , NG Mao-Chu , CHEN Yao-Qiang . Effect of Doping M (M = Mn, Y) into Ce_0.50Zr_0.50O₂ on the Properties of MnO_x/Ce_0.50-zZr_0.50-zM_2zO_y/Al₂O₃ for Catalytic Combustion of Ethyl Acetate. Acta Physico-Chimica Sinica, 2012, 28(08): 1936-1942. doi: 10.3866/PKU.WHXB201205173
9. [9]
  Ming Wang , Min Shao , Si-Hua Lu , Yu-Dong Yang , Wen-Tai Chen . Evidence of coal combustion contribution to ambient VOCs during winter in Beijing. Chinese Chemical Letters, 2013, 24(9): 829-832.
10. [10]
  Shan Huang , Min Shao , Sihua Lu , Ying Liu . Reactivity of ambient volatile organic compounds (VOCs) in summer of 2004 in Beijing. Chinese Chemical Letters, 2008, 19(5): 573-576. doi: 10.1016/j.cclet.2008.03.029
11. [11]
  Wenlang Li , Quanguo Jiang , Didi Li , Zhimin Ao , Taicheng An . Density functional theory investigation on selective adsorption of VOCs on borophene. Chinese Chemical Letters, 2021, 32(9): 2803-2806. doi: 10.1016/j.cclet.2021.01.026
12. [12]
  Sameh M. K. Aboul-Fotouh . Production of dimethylether (DME) as a clean fuel using sonochemically prepared CuO and/or ZnO-modified γ-alumina catalysts. Journal of Fuel Chemistry and Technology, 2014, 42(3): 350-356.
13. [13]
  Fadhil Mustafa H. , Ammar Saad H. , Abdul Jabbar Marwa F. . Microwave-assisted catalytic oxidative desulfurization of gasoil fuel using synthesized CuO-ZnO nanocomposites. Journal of Fuel Chemistry and Technology, 2019, 47(9): 1075-1082.
14. [14]
  Kong Linlin , Jin Xinyi , Hu Dapeng , Feng Leyun , Chen Dong , Li Hanying . Functional delivery vehicle of organic nanoparticles in inorganic crystals. Chinese Chemical Letters, 2019, 30(12): 2351-2354. doi: 10.1016/j.cclet.2019.08.007
15. [15]
  LI Wei-Bin , NG Hao . Recent Progress in the Removal of Volatile Organic Compounds by Catalytic Combustion. Acta Physico-Chimica Sinica, 2010, 26(04): 885-894. doi: 10.3866/PKU.WHXB20100436
16. [16]
  Peng Liu , Chao Long , Hong Ming Qian , Ying Li , Ai Min Li , Quan Xing Zhang . Synthesis and application of a hydrophobic hypercrosslinked polymeric resin for removing VOCs from humid gas stream. Chinese Chemical Letters, 2009, 20(4): 492-495. doi: 10.1016/j.cclet.2008.11.019
17. [17]
  Feng Aihu , Yu Yang , Yu Yun , Song Lixin . Recent Progress in the Removal of Volatile Organic Compounds by Zeolite and Its Supported Catalysts. Acta Chimica Sinica, 2018, 76(10): 757-773. doi: 10.6023/A18060250
18. [18]
  Rui OU , Meng-Ting LIU , Yu-Tong LU , Xu-Yu WANG , Ai-Hua YUAN , Lu-Lu LI , Fu YANG . Improved Catalytic Abatement Efficiency of VOCs via Creating Efficient Synergy of Dispersed Cu-Co Oxides in Molecular Sieve. Chinese Journal of Inorganic Chemistry, 2021, 37(7): 1322-1336. doi: 10.11862/CJIC.2021.146
19. [19]
  Hongyu Liu , Gang Meng , Zanhong Deng , Meng Li , Junqing Chang , Tiantian Dai , Xiaodong Fang . Progress in Research on VOC Molecule Recognition by Semiconductor Sensors. Acta Physico-Chimica Sinica, 2022, 38(5): 2008018-0. doi: 10.3866/PKU.WHXB202008018

Get Citation

PDF

XML

Metrics

PDF Downloads(0)
Abstract views(32)
HTML views(6)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142