Citation: Qingjiang Yu, Kecheng Jiang, Cuiling Yu, Xianjin Chen, Chuanjian Zhang, Yi Yao, Bin Jiang, Huijin Long. Recent progress of composite solid polymer electrolytes for all-solid-state lithium metal batteries[J]. Chinese Chemical Letters, ;2021, 32(9): 2659-2678. doi: 10.1016/j.cclet.2021.03.032 shu

Recent progress of composite solid polymer electrolytes for all-solid-state lithium metal batteries

Qingjiang Yu ^{a, 1} ,
Kecheng Jiang ^{a, 1} ,
Cuiling Yu ^{b, *,} ,
Xianjin Chen ^a ,
Chuanjian Zhang ^a ,
Yi Yao ^a ,
Bin Jiang ^{a, *,} ,
Huijin Long ^{a, *,}

a.
Jiangsu TAFEL New Energy Technology Co., Ltd., Nanjing 211106, China
b.
School of Physics, Harbin Institute of Technology, Harbin 150001, China

Author Bio: Qingjiang Yu received his Ph.D. degree from Jilin University in 2008. Then he joined in Changchun Institute of Applied Chemistry, Chinese Academy of Science, as a postdoctoral researcher. In 2012, he became an associate professor at Harbin Institute of Technology. He joined in TAFEL New Energy Technology Co., Ltd. in 2018. His current research interests are solid-state lithium metal batteries and new materials development for lithium-ion batteries.
Kecheng Jiang received his Ph.D. degree from Institute of Chemistry, Chinese Academy of Sciences, in 2014. He joined TAFEL New Energy Technology Co., Ltd. in 2016. He is now interested in the development of new materials and related technologies for electric vehicle batteries.
Cuiling Yu received his Ph.D. degree from Jilin University in 2008. Then she worked as a senior engineer at Jilin Institute of Metrology. In 2011, she joined in Harbin Institute of Technology. Her current research interests are focused on photoelectrochemical cells and lithium-ion batteries.
Xianjin Chen received his B.S. and M.S. from Shanxi University of Science and Technology in 2014 and 2017, respectively. Then he joined in the Fujian Institute of Research on the Structure, Chinese Academy of Sciences. In 2019, he worked as an engineer at TAFEL New Energy Technology Co., Ltd. He is now interested in solid-state lithium metal batteries.
Chuanjian Zhang received his Ph.D. degree from Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, in 2013. After a 29-months stay as a material engineer in the Watt lab, Huawei Technology, he joined in TAFEL New Energy Technology Co., Ltd. in 2018. His research interests are high-energydensity lithium-ion battery anode materials, such as silicon anode and high capacity artificial graphite.
Yi Yao received his Ph.D. degree from Dalian Institute of Chemistry & Physics, Chinese Academy of Sciences, in 2015. He joined TAFEL New Energy Technology Co., Ltd. in 2018. He is now interested in cathode materials development for lithium-ion batteries.
Bin Jiang received his B.S. and M.S. from Qingdao University of Science and Technology in 2006 and 2009, respectively. Then he joined in Amperex Technology Limited and Contemporary Amperex Technology Co., Ltd. in 2009 and 2011, respectively, studying the lithiumion battery design for electric vehicles. He and his partners established Tafel New Energy Technology Co., Ltd. in 2015. He is now interested in advanced energy materials and their applications in electric vehicle batteries.
Huijin Long received his B.S. and Ph.D. from Jilin University in 2004 and 2009, respectively. He then joined in Changchun institute of applied chemistry Chinese academy of science as a postdoctoral researcher. In 2011, he became an engineer at Contemporary Amperex Technology Co., Ltd., in charge of improving the service life of electric vehicle batteries. He and his partners established Tafel New Energy Technology Co., Ltd. in 2015. His current research interests are focused on in the development of new materials and advanced technologies for electric vehicle batteries.

cuiling.yu@hit.edu.cn

bin.jiang@tafel.com.cn

huijin.long@tafel.com.cn

Received Date: 14 September 2020
Revised Date: 12 January 2021
Accepted Date: 12 March 2021
Available Online: 15 March 2021

Figures(13)

In comparison with lithium-ion batteries (LIBs) with liquid electrolytes, all-solid-state lithium batteries (ASSLBs) have been considered as promising systems for future energy storage due to their safety and high energy density. As the pivotal component used in ASSLBs, composite solid polymer electrolytes (CSPEs), derived from the incorporation of inorganic fillers into solid polymer electrolytes (SPEs), exhibit higher ionic conductivity, better mechanical strength, and superior thermal/electrochemical stability compared to the single-component SPEs, which can significantly promote the electrochemical performance of ASSLBs. Herein, the recent advances of CSPEs applied in ASSLBs are presented. The effects of the category, morphology and concentration of inorganic fillers on the ionic conductivity, mechanical strength, electrochemical window, interfacial stability and possible Li⁺ transfer mechanism of CSPEs will be systematically discussed. Finally, the challenges and perspectives are proposed for the future development of high-performance CSPEs and ASSLBs.
- Composite solid polymer electrolyte,
- All-solid-state lithium battery,
- Ionic conductivity,
- Li⁺ transport,
- Electrochemical property
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沈阳化工大学材料科学与工程学院沈阳 110142