Citation: Fangping Zhuo, Huimin Qiao, Jiaming Zhu, Shuize Wang, Yang Bai, Xinping Mao, Hong-Hui Wu. Perspective on antiferroelectrics for energy storage and conversion applications[J]. Chinese Chemical Letters, ;2021, 32(7): 2097-2107. doi: 10.1016/j.cclet.2020.11.070 shu

Perspective on antiferroelectrics for energy storage and conversion applications

Fangping Zhuo ^{a, b} ,
Huimin Qiao ^c ,
Jiaming Zhu ^{d, *,} ,
Shuize Wang ^{a, *,} ,
Yang Bai ^a ,
Xinping Mao ^a ,
Hong-Hui Wu ^{a, *,}

a.
Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, Beijing 100083, China
b.
Department of Materials and Earth Science, Technical University of Darmstadt, Darmstadt 64287, Germany
c.
School of Advanced Materials and Engineering, Sungkyunkwan University (SKKU), Suwon 16419, Republic of Korea
d.
Department of Mechanical Engineering, The Hong Kong Polytechnic University, Hong Kong, China

zhujiaming@sdu.edu.cn

wangshuize@ustb.edu.cn

wuhonghui@ustb.edu.cn

Received Date: 10 October 2020
Revised Date: 26 November 2020
Accepted Date: 30 November 2020
Available Online: 4 December 2020

Figures(4)

As a close relative of ferroelectricity, antiferroelectricity has received a recent resurgence of interest driven by technological aspirations in energy-efficient applications, such as energy storage capacitors, solid-state cooling devices, explosive energy conversion, and displacement transducers. Though prolonged efforts in this area have led to certain progress and the discovery of more than 100 antiferroelectric materials over the last 70 years, some scientific and technological issues remain unresolved. Herein, we provide perspectives on the development of antiferroelectrics for energy storage and conversion applications, as well as a comprehensive understanding of the structural origin of antiferroelectricity and field-induced phase transitions, followed by design strategies for new lead-free antiferroelectrics. We also envision unprecedented challenges in the development of promising antiferroelectric materials that bridge materials design and real applications. Future research in these directions will open up new possibilities in resolving the mystery of antiferroelectricity, provide opportunities for comprehending structure-property correlation and developing antiferroelectric/ferroelectric theories, and suggest an approach to the manipulation of phase transitions for real-world applications.
- Antiferroelectric materials,
- Energy storage,
- Energy conversion,
- Solid-state cooling,
- Structural origin,
- Phase transition
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