Citation: Xugeng Guo, Wenpeng Wu, Yuanyuan Li, Jinglai Zhang, Wang Li, Hans Ågren. Recent research progress for upconversion assisted dye-sensitized solar cells[J]. Chinese Chemical Letters, ;2021, 32(6): 1834-1846. doi: 10.1016/j.cclet.2020.11.057 shu

Recent research progress for upconversion assisted dye-sensitized solar cells

Xugeng Guo ^{a, b} ,
Wenpeng Wu ^{a, b} ,
Yuanyuan Li ^{a, b} ,
Jinglai Zhang ^{a, b} ,
Wang Li ^{a, b, *,} ,
Hans Ågren ^{a, b, c, *,}

a.
Institute of Upconversion Nanoscale Materials, College of Chemistry and Chemical Engineering, Henan University, Kaifeng 475004, China
b.
Henan Center for Outstanding Overseas Scientists, Henan University, Kaifeng 475004, China
c.
Department of Physics and Astronomy, Uppsala University, Box 516, SE-751 20 Uppsala, Sweden

chemwangl@henu.edu.cn

hagren@kth.se

Received Date: 30 September 2020
Revised Date: 22 November 2020
Accepted Date: 25 November 2020
Available Online: 1 December 2020

Figures(28)

Upconversion (UC) technology makes it possible to harvest infrared (IR) light from the sun and has increasingly been employed in recent years to improve the efficiency of solar cells. The progress in the area concerns both research on fundamental principles and processes of UC and technologies of device fabrication. Significant increase of important solar cell parameters, like short-circuit photocurrent density and open-circuit photovoltage as well as the total photon-to-current efficiency, has been accomplished. We here review the research published during the last few years in the area, in particular we consider the two most cherished techniques, namely the incorporation of upconverting nanophosphors directly into the photoanodes of the solar cells and the introduction of plasmonic metal nanoparticles co-existing with the UC particles. Other ways to achieve strong field enhancement, and the use of the non-linear nature of UC, is to apply microlenses, with or without assisting plasmonic excitation. Further enhanced UC action has been demonstrated by broad band and effective harvesting by organic IR antennas, with subsequent mediation by an intermediate nanoshell of the energy into the upconverting core. Codoping, nanohybrid and layer-by-layer technologies involving upconverting particles as well as the use of upconverting nanoparticles in hole-transport and electrolyte layers, tested in recent works, are also reviewed. While most of these technologies employ upconverting rare earth metals for sequential photon absorption, the main alternative technique, namely triplet-triplet annihilation UC using organic materials, is also reviewed. It is our belief that all these approaches will be further much researched in the near future, with potentially great impact on solar cell technology.
- Upconversion nanoparticles,
- Dye-sensitized solar cells,
- Infrared light,
- Triplet-triplet annihilation,
- Photovoltaic systems
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沈阳化工大学材料科学与工程学院沈阳 110142