Citation: Huang Guihua, Song Xinhong, Chen Yiying, Lin Fangyuan, Huang Yipeng, Li Feiming, Guo Zhiyong, Yao Qiuhong, Chen Xi. Study of the effect of chemical composition on the surface wettability of three-dimensional graphene foams[J]. Chinese Chemical Letters, ;2020, 31(7): 1839-1842. doi: 10.1016/j.cclet.2020.02.053 shu

Study of the effect of chemical composition on the surface wettability of three-dimensional graphene foams

Huang Guihua ^a,1 ,
Song Xinhong ^c,1 ,
Chen Yiying ^b ,
Lin Fangyuan ^b ,
Huang Yipeng ^b ,
Li Feiming ^b ,
Guo Zhiyong ^a ,
Yao Qiuhong ^a ,
Chen Xi ^b,*,

a.
Institute of Analytical Technology and Smart Instruments, College of Environment and Public Health, XiamenHuaxia University, Xiamen 361024, China
b.
State Key Laboratory of Marine Environmental Science, Xiamen University, Xiamen 361005, China
c.
College of Ocean Science and Engineering, Shanghai Maritime University, Shanghai 201306, China

xichen@xmu.edu.cn

Received Date: 4 January 2020
Revised Date: 26 February 2020
Accepted Date: 27 February 2020
Available Online: 28 February 2020

Figures(3)

The chemical composition obviously affects the surface wettability of a three-dimensional (3D) graphene material apart from its surface energy and microstructure. In the hydrothermal preparation, the heteroatom doping changes the chemical composition and wettability of the 3D graphene material. To realize the controllable surface wettability of graphene materials, aminobenzene sulfonic acid (ABSA) was selected as a typical doping agent for the preparation of nitrogen and sulfur co-doped 3D graphene foam (SNGF) using a hydrothermal method. Different from using o-ABSA or p-ABSA as the dopant, SNGF with tunable surface wettability is obtained only when m-ABSA is used. This result indicates that the substituent position of -SO₃H group in the benzene ring of ABSA is rather important for the tunable wettability. This work provides some theoretical foundations for dopant selection and some new insights in manipulating the properties of 3D graphene foams by adjusting the configuration of dopants.
- 3D graphene foam,
- Surface wettability,
- Dopant configuration,
- Chemical composition,
- Aminobenzene sulfonic acid
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