Citation: Zhang Chao, Li Tingting, Pu Lei, Wen Weijia, Luo Xiangdong, hao LijuanZ. Enhanced photoluminescence and stability of ZnSe microspheres/Cs₄PbBr₆ microcrystals/CsPbBr₃ nanocrystals composites[J]. Chinese Chemical Letters, ;2020, 31(9): 2499-2502. doi: 10.1016/j.cclet.2020.01.013 shu

Enhanced photoluminescence and stability of ZnSe microspheres/Cs₄PbBr₆ microcrystals/CsPbBr₃ nanocrystals composites

Zhang Chao ^a,b,c ,
Li Tingting ^a,c ,
Pu Lei ^a,c ,
Wen Weijia ^a ,
Luo Xiangdong ^b ,
hao LijuanZ ^a,c,*,

a.
Materials Genome Institute, Shanghai University, Shanghai 200444, China
b.
Jiangsu Key Laboratory of ASIC Design, Nantong University, Nantong 226019, China
c.
State Key Laboratory of Transducer Technology, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai 200050, China

zhaolijuan@t.shu.edu.cn

Received Date: 16 December 2019
Revised Date: 2 January 2020
Accepted Date: 7 January 2020
Available Online: 9 January 2020

Figures(4)

A ternary complex combining dual-phase perovskites - Cs₄PbBr₆/CsPbBr₃ (DP-CPB) with ZnSe micropsheres (ZnSe-DP-CPB) was successfully prepared using supersaturated recrystallization technique at room temperature. It was showed that the DP-CPB composites were partially embedded in ZnSe microsphere composed with ZnSe NCs. The light absorption range of ZnSe-DP-CPB composites was extended from visible to near infrared light. Highly enhanced luminescence from ZnSe-DP-CPB composite was observed and the excitation power-dependent photoluminescence showed that the recombination involves excitons. The recombination lifetimes of the ternary composites increased compared with DP-CPB composite, indicating that the non-radiative combination was suppressed which may be possibly due to the decrease of both bulk and surface defects, owing to the passivation of ZnSe, as well as the suitable band alignments of these three components. The ternary complex also showed improved stability of photoluminescence (PL), which opens a new avenue for enhancing the stability of PL and optoelectronic applications for semiconductor-perovskite composites.
- Dual-phase perovskites,
- Ternary complex,
- Supersaturated recrystallization,
- Photoluminescence,
- Passivation,
- Optoelectronic
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Enhanced photoluminescence and stability of ZnSe microspheres/Cs₄PbBr₆ microcrystals/CsPbBr₃ nanocrystals composites