Citation: Ding Yongqiang, Li Yali, Li Junshuai, Yan Xingbin. High-performance nitrogen and sulfur co-doped nanotube-like carbon anodes for sodium ion hybrid capacitors[J]. Chinese Chemical Letters, ;2020, 31(9): 2219-2224. doi: 10.1016/j.cclet.2019.11.017 shu

High-performance nitrogen and sulfur co-doped nanotube-like carbon anodes for sodium ion hybrid capacitors

Ding Yongqiang ^a ,
Li Yali ^a,*, ,
Li Junshuai ^a,*, ,
Yan Xingbin ^b

a.
Key Laboratory of Special Function Materials & Structure Design of the Ministry of Education, School of Physical Science & Technology, Lanzhou University, Lanzhou 730000, China
b.
Laboratory of Clean Energy Chemistry and Materials, State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China

liyli@lzu.edu.cn

jshli@lzu.edu.cn

Received Date: 18 September 2019
Revised Date: 5 November 2019
Accepted Date: 11 November 2019
Available Online: 13 November 2019

Figures(6)

Sodium ion hybrid capacitors are of great concern in large-scale and cost-effective electrical energy storage owing to their high energy and power densities, as well as natural abundance and wide distribution of sodium. However, it is difficult to find a well-pleasing anode material that matches the high-performance cathode materials to achieve good energy and power output for sodium ion hybrid capacitors. In this paper, nitrogen and sulfur co-doped nanotube-like carbon prepared by a simple carbonization process of high sulfur-loaded polyaniline nanotubes is introduced as the anode. The assembled sodium ion half cell based on the optimal nanotube-like carbon delivers a high reversible capacity of ~304.8 mAh/g at 0.2 A/g and an excellent rate performance of ~124.8 mAh/g at 10 A/g in a voltage window of 0.01-2.5 V (versus sodium/sodium ion). For the hybrid capacitors assembled using the optimal nanotube-like carbon as the anode and high-capacity activated carbon as the cathode, high energy densities of ~100.2 Wh/kg at 250 W/kg and ~50.69 Wh/kg at 12, 500 W/kg are achieved.
- Sodium ion hybrid capacitors,
- Anode,
- Nanotube-like carbon,
- Polyaniline nanotubes,
- Electrical energy storage
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