Citation: Yang Yulu, Tang Yang, Jiang Haomin, Chen Yongmei, Wan Pingyu, Fan Maohong, Zhang Rongrong, Ullah Sana, Pan Lun, Zou Ji-Jun, Lao Mengmeng, Sun Wenping, Yang Chao, Zheng Gengfeng, Peng Qiling, Wang Ting, Luo Yonglan, Sun Xuping, Konev Alexander S., Levin Oleg V., Lianos Panagiotis, Hu Zhuofeng, Shen Zhurui, Zhao Qinglan, Wang Ying, Todorova Nadia, Trapalis Christos, Sheridan Matthew V., Wang Haipeng, Zhang Ling, Sun Songmei, Wang Wenzhong, Ma Jianmin. 2020 Roadmap on gas-involved photo-and electro-catalysis[J]. Chinese Chemical Letters, ;2019, 30(12): 2089-2109. doi: 10.1016/j.cclet.2019.10.041 shu

2020 Roadmap on gas-involved photo-and electro-catalysis

Yang Yulu ^a ,
Tang Yang ^b ,
Jiang Haomin ^b ,
Chen Yongmei ^b, ,
Wan Pingyu ^b ,
Fan Maohong ^c,d,**, ,
Zhang Rongrong ^e,f ,
Ullah Sana ^e,f ,
Pan Lun ^e,f ,
Zou Ji-Jun ^e,f, ,
Lao Mengmeng ^g ,
Sun Wenping ^g, ,
Yang Chao ^h ,
Zheng Gengfeng ^h, ,
Peng Qiling ⁱ ,
Wang Ting ^i,j ,
Luo Yonglan ^j ,
Sun Xuping ^i, ,
Konev Alexander S. ^k ,
Levin Oleg V. ^k, ,
Lianos Panagiotis ^l, ,
Hu Zhuofeng ^m, ,
Shen Zhurui ^n, ,
Zhao Qinglan ^o ,
Wang Ying ^o, ,
Todorova Nadia ^p ,
Trapalis Christos ^p, ,
Sheridan Matthew V. ^q, ,
Wang Haipeng ^r,s ,
Zhang Ling ^r,s ,
Sun Songmei ^r,s ,
Wang Wenzhong ^r,s, ,
Ma Jianmin ^a,t,*,

a.
School of Physics and Electronics, Hunan University, Changsha 410082, China
b.
College of Chemistry, Beijing University of Chemical Technology, Beijing 100029, China
c.
School of Civil and Environmental Engineering, Georgia Institute of Technology, Atlanta, GA 30332, United States
d.
College of Engineering and Applied Sciences, and School of Energy Resources, University of Wyoming, Laramie, WY 82071, United States
e.
Key Laboratory for Green Chemical Technology of the Ministry of Education, School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China
f.
Collaborative Innovative Center of Chemical Science and Engineering(Tianjin), Tianjin 300072, China
g.
Institute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, Wollongong, NSW 2522, Australia
h.
Laboratory of Advanced Materials, Department of Chemistry, Fudan University, Shanghai 200438, China
i.
Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China
j.
Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province, College of Chemistry and Chemical Engineering, China West Normal University, Nanchong 637002, China
k.
Institute of Chemistry, St. Petersburg State University, 7/9 Universitetskaya emb., St. Petersburg 199034, Russian Federation
l.
Department of Chemical Engineering, University of Patras, Patras 26500, Greece
m.
School of Environmental Science and Engineering, Guangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology, Sun Yat-sen University, Guangzhou 510275, China
n.
School of Materials Science and Engineering, Nankai University, Tianjin 300350, China
o.
Department of Chemistry, Chinese University of Hong Kong, Hong Kong, China
p.
Institute of Nanoscience and Nanotechnology, NCSR "Demokritos", Athens 15341, Greece
q.
State Key Laboratory of School of Radiation Medicine and Protection and School for Radiological and interdisciplinary Sciences(RAD-X), Soochow University, Suzhou 215123, China
r.
State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China
s.
Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
t.
Key Laboratory of Materials Processing and Mold(Zhengzhou University), Ministry of Education, Zhengzhou University, Zhengzhou 450002, China

^**

chenym@mail.buct.edu.cn

huzhf8@mail.sysu.edu.cn

shenzhurui@tju.edu.cn

ying.b.wang@cuhk.edu.hk

c.trapalis@inn.demokritos.gr

Matt1@suda.edu.cn

wzwang@mail.sic.ac.cn

nanoelechem@hnu.edu.cn

Received Date: 20 August 2019
Revised Date: 5 October 2019
Accepted Date: 31 October 2019
Available Online: 9 December 2019

Figures(12)

Green reactions not only provide us chemical products without any pollution, but also offer us the viable technology to realize difficult tasks in normal conditions. Photo-, photoelectro-, and electrocatalytic reactions are indeed powerful tools to help us to embrace bright future. Especially, some gas-involved reactions are extremely useful to change our life environments from energy systems to liquid fuels and cost-effective products, such as H₂ evolution (H₂ production), O₂ evolution/reduction, CO₂ reduction, N₂ reduction (or N₂ fixation) reactions. We can provide fuel cells clean H₂ for electric vehicles from H₂ evolution reaction (HER), at the same time, we also need highly efficient O₂ reduction reaction (ORR) in fuel cells for improving the reaction kinetics. Moreover, we can get the clean oxidant O₂ from water through O₂ evolution reaction (OER), and carry out some reactions without posing any pollution to reaction systems. Furthermore, we can translate the greenhouse gas CO₂ into useful liquid fuels through CO₂ reduction reaction (CRR). Last but not the least, we can get ammonia from N₂ reduction reaction (NRR), which can decrease energy input compared to the traditional Hubble process. These reactions, such as HER, ORR, OER, CRR and NRR could be realized through solar-, photoelectro-and electro-assisted ways. For them, the catalysts used play crucial roles in determining the efficiency and kinds of products, so we should consider the efficiency of catalysts. However, the cost, synthetic methods of catalysts should also be considered. Nowadays, significant progress has been achieved, however, many challenges still exist, reaction systems, catalysts underlying mechanisms, and so on. As extremely active fields, we should pay attention to them. Under the background, it has motivated us to contribute with a roadmap on 'GasInvolved Photo-and Electro-Catalysis'.
- H₂ evolution reaction,
- O₂ reduction reaction,
- O₂ evolution reaction,
- CO₂ reduction reaction,
- N₂ reduction reaction,
- Electrocatalysis,
- Photocatalysis,
- Photoelectrocatalysis
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