Citation: An Pan, Kang Longtian, Tang Zhen, Su Peifeng, Luo Zhixun. Spectroscopic identification towards tunable mesoscale aggregates of zinc tetraphenylporphyrin for materials[J]. Chinese Chemical Letters, ;2018, 29(3): 361-365. doi: 10.1016/j.cclet.2017.11.009 shu

Spectroscopic identification towards tunable mesoscale aggregates of zinc tetraphenylporphyrin for materials

An Pan ^a ,
Kang Longtian ^b ,
Tang Zhen ^c ,
Su Peifeng ^c,, ,
Luo Zhixun ^a,,

a.
State Key Laboratory for Structural Chemistry of Unstable and Stable Species, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
b.
Fujian Institute of Research on the Structure of Matter Fujian, Chinese Academy of Sciences, Fuzhou 350002, China
c.
State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China

Corresponding author: Su Peifeng, supi@xmu.edu.cn Luo Zhixun, jielilzx@iccas.ac.cn; zxluo@iccas.ac.cn
Received Date: 7 September 2017
Revised Date: 7 November 2017
Accepted Date: 7 November 2017
Available Online: 10 March 2017

Figures(4)

We present a study of spectroscopic identification towards the molecular aggregates of zinc tetraphenylporphyrin (ZnTPP) illustrating how the energy states and intermolecular interactions determine the tunable properties of functional materials in condensation processes. Distinguishable fingerprints of ZnTPP nanorods and nanosheets are addressed utilizing X-ray diffraction (XRD), Raman and UV-vis absorption spectroscopies. Although these ZnTPPs are assigned to J-aggregation at different extent, the spectral analysis reveals a significant role of the intermolecular interactions associated with varying mesoscale architectures. Energy decomposition analysis (EDA) revealed that the varied ZnTPP aggregates are stabilized by altered dispersion interactions due to the dominant π…π stacking between the monomers.
- ZnTPP,
- Molecular aggregates,
- Intermolecular interactions,
- Ramanspectroscopy,
- XRD
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