Citation: Gao Nuonuo, Ma Kui, Ding Tong, Cai Jinmeng, Tian Ye, Li Xingang. Enhanced carbon dioxide adsorption performance and kinetic study of K and Al co-doped Li₄SiO₄[J]. Chinese Chemical Letters, ;2018, 29(3): 482-484. doi: 10.1016/j.cclet.2017.07.031 shu

Enhanced carbon dioxide adsorption performance and kinetic study of K and Al co-doped Li₄SiO₄

Collaborative Innovation Center for Chemical Science & Engineering(Tianjin), Tianjin Key Laboratory of Applied Catalysis Science & Engineering, School of Chemical Engineering & Technology, Tianjin University, Tianjin 30072, China

Corresponding author: Ding Tong, d_tong@tju.edu.cn Li Xingang, xingang_li@tju.edu.cn
Received Date: 26 April 2017
Revised Date: 20 May 2017
Accepted Date: 30 July 2017
Available Online: 3 March 2017

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Herein, we report the effects of doped K and Al on the carbon dioxide (CO₂) adsorption performance of the Li₄SiO₄-based adsorbents. The CO₂ adsorption capacity of 0.8 wt% K and 1.5 wt% Al doped Li₄SiO₄ is~2.2 times and~1.3 times higher than that of the pristine Li₄SiO₄ at 500 and 600℃, respectively. The kinetic study further indicated that the reaction rates of the lithium diffusion process is greatly improved by K and Al doping, and the lithium diffusion rate of 0.8 wt% K and 1.5 wt% Al doped Li₄SiO₄ is~2 times higher than that of the pristine Li₄SiO₄ at 575-650℃. K and Al doping increases the adsorption capacity of Li₄SiO₄-based adsorbents, and widens its effective adsorption temperature range
- Li₄SiO,
- K and Al doping,
- CO₂ adsorption,
- Kinetic study,
- Adsorption stability
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Enhanced carbon dioxide adsorption performance and kinetic study of K and Al co-doped Li₄SiO₄