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嵌入镍纳米颗粒的生物相容性空心碳纳米纤维中应变梯度与表面应力介导的电磁吸收

高峰 ,  郭雨鑫 ,  刘雲龙 ,  李圣元 ,  李海丰 ,  李佳兴 ,  李赛楠 ,  赵永鹏 ,  贺改花 ,  任振堃

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引用本文: 高峰, 郭雨鑫, 刘雲龙, 李圣元, 李海丰, 李佳兴, 李赛楠, 赵永鹏, 贺改花, 任振堃. 嵌入镍纳米颗粒的生物相容性空心碳纳米纤维中应变梯度与表面应力介导的电磁吸收[J]. 物理化学学报, 2026, 42(11): 100407. doi: 10.1016/j.actphy.2026.100407 shu
Citation:  Feng Gao,  Yuxin Guo,  Yunlong Liu,  Shengyuan Li,  Haifeng Li,  Jiaxin Li,  Sainan Li,  Yongpeng Zhao,  Gaihua He,  Zhenkun Ren. 嵌入镍纳米颗粒的生物相容性空心碳纳米纤维中应变梯度与表面应力介导的电磁吸收[J]. Acta Physico-Chimica Sinica, 2026, 42(11): 100407. doi: 10.1016/j.actphy.2026.100407 shu

嵌入镍纳米颗粒的生物相容性空心碳纳米纤维中应变梯度与表面应力介导的电磁吸收

  • 1.

    锦州医科大学附属第三医院, 辽宁锦州 121000;

  • 2.

    锦州医科大学药学院, 辽宁 锦州 121000;

  • 3.

    四川农业大学机电工程学院, 四川雅安 625000;

  • 4.

    中国医科大学药学院, 辽宁 沈阳 110122;

  • 5.

    湖北汽车工业学院汽车材料学院, 湖北十堰 442002

    • 通讯作者: 赵永鹏,E-mail:zhaoyp@sicau.edu.cn; 贺改花,E-mail:ghHe2020@yeah.net; 任振堃,E-mail:renzk@jzmu.edu.cn
  • 基金项目:

    本研究得到辽宁省科技计划联合项目(2024012152-JH4/4800，2024-MSLH-155)；国家自然科学基金(52402293，52402118)以及四川省自然科学基金(2026NSFSC0358)的支持。

摘要: 开发兼具强衰减能力和良好生物相容性的高性能电磁波(EMW)吸收材料，对于可穿戴电子、植入式设备和便携式医疗设备等新兴应用日益重要。本研究通过静电纺丝结合牺牲模板法及后续高温碳化，制备了一类具有精确曲率控制的中空磁性碳纳米纤维(Ni/HCNFs)调节SiO2米球的直径，系统调控了纳米纤维的内部空腔尺寸和几何曲率。优化后的具有300 nm空腔的Ni/HCNFs表现出优异的反射损耗最小值-58.7 dB和有效吸收带宽5.28 GHz。增强的电磁波吸收归因于阻抗匹配优化、中空空腔内多次反射以及由曲率诱导的晶格应变梯度和表面应力场引起的界面/偶极极化损耗增强的协同效应，这已通过密度泛函理论计算和有限元模拟得到验证。此外，初步生物相容性评估表明，Ni/HCNFs在与成纤维细胞共培养时表现出低细胞毒性和良好的细胞活力，表明其作为未来生物集成电子系统中安全高效的电磁波吸收材料的潜力。这项工作不仅为设计轻质高性能电磁波吸收材料提供了稳健策略，也为它们在生物相容性、靶向微波热疗载体和环境适应性场景中的应用开辟了新途径。

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