双限域基质实现千克级连续可调白色室温磷光碳点复合材料

引用本文: 胡新洲, 朱传奇, 康艺红, 石林林, 张永强, 卢思宇. 双限域基质实现千克级连续可调白色室温磷光碳点复合材料[J]. 物理化学学报, 2026, 42(11): 100369. doi: 10.1016/j.actphy.2026.100369 shu

Citation: Xinzhou Hu, Chuanqi Zhu, Yihong Kang, Linlin Shi, Yongqiang Zhang, Siyu Lu. 双限域基质实现千克级连续可调白色室温磷光碳点复合材料[J]. Acta Physico-Chimica Sinica, 2026, 42(11): 100369. doi: 10.1016/j.actphy.2026.100369 shu

双限域基质实现千克级连续可调白色室温磷光碳点复合材料

胡新洲 ^1, ,
朱传奇 ^1, ,
康艺红 ^1, ,
石林林 ^{1,
,} ,
张永强 ^{1,
,} ,
卢思宇 ^{1,2,
,}

1.
郑州大学化学学院平原实验室, 河南郑州 450001;
2.
抗病毒性传染病创新药物全国重点实验室(河南大学), 河南郑州 450046

通讯作者: 石林林,E-mail:linlinshi@zzu.edu.cn; 张永强,E-mail:zhangyongqiang@zzu.edu.cn; 卢思宇,E-mail:sylu2013@zzu.edu.cn

基金项目:
本研究得到了国家自然科学基金(U24A2079和22575225)、河南省自然科学基金(242300421068和232301420006)以及中国博士后科学基金(2025T180303)的资助。

摘要: 本研究创新性地提出了一种基质比例调控策略，通过一步水热法合成了可调谐白色室温磷光(RTP)碳点嵌入三氧化二硼(B₂O₃)与三聚氰酸(CA)双限域复合材料(记为W-CD@B₂O₃-CA)。通过调节基质比例并利用多重限域效应，所获得的W-CD@B₂O₃-CA实现了从暖白光到中性白光、再到冷白光的宽范围色度调控，显色指数从85.6提升至91.1。系统表征表明，白色余辉发射源于碳核尺寸、表面官能团及基质内B/N共掺杂的协同贡献。基于其独特的光学特性，成功开发了高对比度指纹识别与多级信息加密应用。此外，通过优化合成工艺，实现了低成本、高产率的公斤级制备，为新型高效白色RTP材料的实际探索提供了新路径。

关键词:

English

双限域基质实现千克级连续可调白色室温磷光碳点复合材料

Xinzhou Hu ^1, ,
Chuanqi Zhu ^1, ,
Yihong Kang ^1, ,
Linlin Shi ^{1,
,} ,
Yongqiang Zhang ^{1,
,} ,
Siyu Lu ^{1,2,
,}

1.
College of Chemistry, Pingyuan Laboratory, Zhengzhou University, Zhengzhou 450001, Henan Province, China;
2.
State Key Laboratory of Antiviral Drugs, Henan University, Zhengzhou 450046, Henan Province, China

Corresponding author: Linlin Shi, ; Yongqiang Zhang, ; Siyu Lu,

Received Date: 28 May 2026
Accepted Date: 13 July 2026
Revised Date: 08 July 2026

Abstract: 本研究创新性地提出了一种基质比例调控策略，通过一步水热法合成了可调谐白色室温磷光(RTP)碳点嵌入三氧化二硼(B₂O₃)与三聚氰酸(CA)双限域复合材料(记为W-CD@B₂O₃-CA)。通过调节基质比例并利用多重限域效应，所获得的W-CD@B₂O₃-CA实现了从暖白光到中性白光、再到冷白光的宽范围色度调控，显色指数从85.6提升至91.1。系统表征表明，白色余辉发射源于碳核尺寸、表面官能团及基质内B/N共掺杂的协同贡献。基于其独特的光学特性，成功开发了高对比度指纹识别与多级信息加密应用。此外，通过优化合成工艺，实现了低成本、高产率的公斤级制备，为新型高效白色RTP材料的实际探索提供了新路径。

Key words:

Tunable white-light afterglow carbon dots composites
/ Kilogram-scale synthesis
/ Multiple confinement effects
/ Fingerprint imaging
/ Information encryption

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沈阳化工大学材料科学与工程学院沈阳 110142

双限域基质实现千克级连续可调白色室温磷光碳点复合材料

通讯作者: 石林林,E-mail:linlinshi@zzu.edu.cn; 张永强,E-mail:zhangyongqiang@zzu.edu.cn; 卢思宇,E-mail:sylu2013@zzu.edu.cn

English

双限域基质实现千克级连续可调白色室温磷光碳点复合材料

Corresponding author: Linlin Shi, ; Yongqiang Zhang, ; Siyu Lu,

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中国化学会秘书处

双限域基质实现千克级连续可调白色室温磷光碳点复合材料

通讯作者: 石林林,E-mail:linlinshi@zzu.edu.cn; 张永强,E-mail:zhangyongqiang@zzu.edu.cn; 卢思宇,E-mail:sylu2013@zzu.edu.cn

English

双限域基质实现千克级连续可调白色室温磷光碳点复合材料

Corresponding author: Linlin Shi, ; Yongqiang Zhang, ; Siyu Lu,

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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