MoS<sub>2</sub>调控TiO<sub>2</sub>/C形成介电损耗主导的绣球花结构用于电磁波吸收

引用本文: 胡玉鹏, 董赛佳, 周腾, 马东威, 张道海, 夏华森, 司元靖, 宋安敏, 徐国敏. MoS₂调控TiO₂/C形成介电损耗主导的绣球花结构用于电磁波吸收[J]. 物理化学学报, 2026, 42(11): 100345. doi: 10.1016/j.actphy.2026.100345 shu

Citation: Yupeng Hu, Saijia Dong, Teng Zhou, Dongwei Ma, Daohai Zhang, Huasen Xia, Yuanjing Si, Anmin Song, Guomin Xu. MoS₂调控TiO₂/C形成介电损耗主导的绣球花结构用于电磁波吸收[J]. Acta Physico-Chimica Sinica, 2026, 42(11): 100345. doi: 10.1016/j.actphy.2026.100345 shu

MoS₂调控TiO₂/C形成介电损耗主导的绣球花结构用于电磁波吸收

胡玉鹏 ^1, ,
董赛佳 ^1, ,
周腾 ^1, ,
马东威 ^2, ,
张道海 ^{1,
,} ,
夏华森 ^1, ,
司元靖 ^1, ,
宋安敏 ^{1,
,} ,
徐国敏 ^{1,
,}

1.
贵州民族大学化学工程学院, 贵州贵阳 550025;
2.
湖北汽车工业学院汽车材料学院, 湖北十堰 442002

通讯作者: 张道海,E-mail:zhangdaohai6235@163.com; 宋安敏,E-mail:songanmin0919@163.com; 徐国敏,E-mail:410034801@qq.com

基金项目:
本研究由国家自然科学基金项目(52163001)；贵州省科技计划项目(黔科合平台人才-GCC[2022]010–2)；中央引导地方科技发展专项资金(黔科合中引地[2024]042、黔科合中引地[2025]013、黔科合人才XKBF[2025]005)；贵州民族大学博士启动基金项目(GZMUZK[2024]QD77)；贵州省科学家工作站(黔科合平台KXJZ[2024]022)；贵州省教育厅“百校千企科技攻关揭榜挂帅”(黔教技[2025]007号)；大学生创新创业训练计划项目(202510672646)共同资助。

摘要: 对于非磁性MOF(金属有机框架)衍生物而言，当前研究的核心挑战在于如何在不引入磁性组分的前提下，通过精确调控材料微观形貌与介电常数来克服阻抗失配并提升吸波性能。引入具有半导体特性与层状结构的二维材料MoS₂可显著增强此类材料的吸收性能。本工作通过在Ti-MOFs上原位生长不同负载量的MoS₂，设计出具有绣球花形貌的新型Ti-MOF衍生物吸波材料(TiO₂/C@MoS₂)以解决上述问题。具体而言，TiO₂/C@MoS₂复合材料TM72在2.05 mm厚度时实现-62.1 dB的最小反射损耗(RL_min)，最大有效吸收带宽(EAB_max)达5.88 GHz (对应厚度2.18 mm)，雷达散射截面(RCS)减缩值为16.6 dB m²；TM71则在匹配厚度2.47 mm时RL_min为-52.82 dB，对应匹配厚度2.28 mm的EAB_max达6.93 GHz，同时实现17.95 dB m²的雷达散射截面(RCS)减缩。这使得TiO₂/C@MoS₂能够满足电磁波吸收材料(EMWAMs)“强、宽、薄、轻”的关键需求。此外，RCS模拟验证了该复合材料的实际适用性。因此，本研究为构建具有超薄结构、优异吸收性能与宽频吸收能力的下一代EMWAMs提供了创新策略。

关键词:

English

MoS₂调控TiO₂/C形成介电损耗主导的绣球花结构用于电磁波吸收

Yupeng Hu ^1, ,
Saijia Dong ^1, ,
Teng Zhou ^1, ,
Dongwei Ma ^2, ,
Daohai Zhang ^{1,
,} ,
Huasen Xia ^1, ,
Yuanjing Si ^1, ,
Anmin Song ^{1,
,} ,
Guomin Xu ^{1,
,}

1.
School of Chemical Engineering, Guizhou Minzu University, Guiyang 550025, Guizhou Province, China;
2.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China

Corresponding author: Daohai Zhang, ; Anmin Song, ; Guomin Xu,

Received Date: 12 April 2026
Accepted Date: 09 June 2026
Revised Date: 07 June 2026

Abstract: 对于非磁性MOF(金属有机框架)衍生物而言，当前研究的核心挑战在于如何在不引入磁性组分的前提下，通过精确调控材料微观形貌与介电常数来克服阻抗失配并提升吸波性能。引入具有半导体特性与层状结构的二维材料MoS₂可显著增强此类材料的吸收性能。本工作通过在Ti-MOFs上原位生长不同负载量的MoS₂，设计出具有绣球花形貌的新型Ti-MOF衍生物吸波材料(TiO₂/C@MoS₂)以解决上述问题。具体而言，TiO₂/C@MoS₂复合材料TM72在2.05 mm厚度时实现-62.1 dB的最小反射损耗(RL_min)，最大有效吸收带宽(EAB_max)达5.88 GHz (对应厚度2.18 mm)，雷达散射截面(RCS)减缩值为16.6 dB m²；TM71则在匹配厚度2.47 mm时RL_min为-52.82 dB，对应匹配厚度2.28 mm的EAB_max达6.93 GHz，同时实现17.95 dB m²的雷达散射截面(RCS)减缩。这使得TiO₂/C@MoS₂能够满足电磁波吸收材料(EMWAMs)“强、宽、薄、轻”的关键需求。此外，RCS模拟验证了该复合材料的实际适用性。因此，本研究为构建具有超薄结构、优异吸收性能与宽频吸收能力的下一代EMWAMs提供了创新策略。

Key words:

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沈阳化工大学材料科学与工程学院沈阳 110142

MoS₂调控TiO₂/C形成介电损耗主导的绣球花结构用于电磁波吸收

通讯作者: 张道海,E-mail:zhangdaohai6235@163.com; 宋安敏,E-mail:songanmin0919@163.com; 徐国敏,E-mail:410034801@qq.com

English

MoS₂调控TiO₂/C形成介电损耗主导的绣球花结构用于电磁波吸收

Corresponding author: Daohai Zhang, ; Anmin Song, ; Guomin Xu,

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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中国化学会秘书处

MoS2调控TiO2/C形成介电损耗主导的绣球花结构用于电磁波吸收

通讯作者: 张道海,E-mail:zhangdaohai6235@163.com; 宋安敏,E-mail:songanmin0919@163.com; 徐国敏,E-mail:410034801@qq.com

English

MoS2调控TiO2/C形成介电损耗主导的绣球花结构用于电磁波吸收

Corresponding author: Daohai Zhang, ; Anmin Song, ; Guomin Xu,

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

MoS₂调控TiO₂/C形成介电损耗主导的绣球花结构用于电磁波吸收

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